Applicability of condensation particle counters to measure atmospheric clusters
This study presents an evaluation of a pulse height condensation particle counter (PH-CPC) and an expansion condensation particle counter (E-CPC) in terms of measuring ambient and laboratory-generated molecular and ion clusters. Ambient molecular cluster concentrations were measured with both instruments as they were deployed in conjunction with an ion spectrometer and other aerosol instruments in Hyytiälä, Finland at the SMEAR II station between 1 March and 30 June 2007. The observed cluster concentrations varied and ranged from some thousands to 100 000 cm -3. Both instruments showed similar (within a factor of ~5) concentrations. An average size of the detected clusters was approximately 1.8 nm. As the atmospheric measurement of sub 2-nm particles and molecular clusters is a challenging task, we conclude that most likely we were unable to detect the smallest clusters. Nevertheless, the reported concentrations are the best estimates to date for minimum cluster concentrations in a boreal forest environment.
|Author:||Mikko Sipilä, Katrianne Lehtipalo, Heikki Junninen, Tuukka Petäjä, Markku Kulmala, Pasi Aalto, Hanna Manninen, Ella-Maria Kyrö, Eija Asmi, Ilona Riipinen, Joachim Curtius, Andreas Kürten, Stephan Borrmann, Colin D. O'Dowd|
|Parent Title (English):||Atmospheric chemistry and physics|
|Publisher:||European Geosciences Union|
|Place of publication:||Katlenburg-Lindau|
|Date of Publication (online):||25.07.2008|
|Date of first Publication:||25.07.2008|
|Publishing Institution:||Univ.-Bibliothek Frankfurt am Main|
|Dewey Decimal Classification:||550 Geowissenschaften|
© Author(s) 2008. This work is distributed under the Creative Commons Attribution 3.0 License.
|Licence (German):||Creative Commons - Namensnennung 3.0|