Mean age of stratospheric air derived from AirCore observations

  • Mean age of stratospheric air can be derived from observations of sufficiently long lived trace gases with approximately linear trends in the troposphere. Mean age can serve as a tracer to investigate stratospheric transport and long term changes in the strength of the overturning Brewer-Dobson circulation of the stratosphere. For this purpose, a low-cost method is required in order to allow for regular observations up to altitudes of about 30 km. Despite the desired low costs, high precision and accuracy are required in order to allow determination of mean age. We present balloon borne AirCore observations from two mid latitude sites: Timmins in Ontario/Canada and Lindenberg in Germany. During the Timmins campaign five AirCores sampled air in parallel from a large stratospheric balloon and were analysed for CO2, CH4 and partly CO. We show that there is good agreement between the different AirCores (better than 0.1 %) especially when vertical gradients are small. The measurements from Lindenberg were performed using small low-cost balloons and yielded very comparable results. We have used the observations to extend our long term data set of mean age observations at Northern Hemi-sphere mid latitudes. The time series now covers more than 40 years and shows a small, statis-tically not significant positive trend of 0.15 ± 0.18 years/decade. This trend is slightly smaller than the previous estimate of 0.24 ± 0.22 years/decade which was based on observations up to the year 2006. These observations are still in contrast to strong negative trends of mean age as derived from some model calculations.

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Author:Andreas EngelORCiD, Harald BönischORCiDGND, Markus Ullrich, Robert Sitals, Olivier Membrive, François Danis, Cyril Crevoisier
URN:urn:nbn:de:hebis:30:3-429275
DOI:https://doi.org/10.5194/acp-2017-104
ISSN:1680-7375
Parent Title (English):Atmospheric chemistry and physics. Discussions
Publisher:European Geosciences Union
Place of publication:Katlenburg-Lindau.
Document Type:Article
Language:English
Year of Completion:2017
Date of first Publication:2017/02/08
Publishing Institution:Universitätsbibliothek Johann Christian Senckenberg
Release Date:2017/02/27
Issue:104
Page Number:36
First Page:1
Last Page:36
Note:
© Author(s) 2017. This work is distributed under the Creative Commons Attribution 3.0 License.
HeBIS-PPN:44631658X
Institutes:Geowissenschaften / Geographie / Geowissenschaften
Dewey Decimal Classification:5 Naturwissenschaften und Mathematik / 55 Geowissenschaften, Geologie / 550 Geowissenschaften
Sammlungen:Universitätspublikationen
Licence (German):License LogoCreative Commons - Namensnennung 3.0