Photoelectron circular dichroism (PECD) was investigated for methyloxirane with intense few-cycle pulses. The observed PECD shows a dependence on electron energy. This may signify an influence of the chiral potential on the outgoing electron’s trajectory.
We introduce and employ the molecular attoclock method. This allows us to simultaneously trace the nuclear and electron dynamics during H2 fragmentation, and to CEP-control the two-electron emission dynamics on sub-cycle time scales.
We demonstrate two-dimensional control over the chargelocalization in H2 dissociation using elliptically polarized laser pulses. The influences of the CEP and the laser phase at the instant of ionization are investigated.