We introduce and employ the molecular attoclock method. This allows us to simultaneously trace the nuclear and electron dynamics during H2 fragmentation, and to CEP-control the two-electron emission dynamics on sub-cycle time scales.
Photoelectron circular dichroism (PECD) was investigated for methyloxirane with intense few-cycle pulses. The observed PECD shows a dependence on electron energy. This may signify an influence of the chiral potential on the outgoing electron’s trajectory.
We demonstrate two-dimensional control over the chargelocalization in H2 dissociation using elliptically polarized laser pulses. The influences of the CEP and the laser phase at the instant of ionization are investigated.