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Year of publication
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- Article (897) (remove)
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Keywords
- Climate change (7)
- climate change (7)
- COSMO-CLM (6)
- Palaeoclimate (6)
- Atmospheric chemistry (5)
- Biogeochemistry (5)
- Palaeoceanography (5)
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In meinen Diluvialstudien 1 und 2 habe ich u.a. den Nachweis zu führen gesucht, dass das Herzogtum Oldenburg nur während der ersten Glacialperiode vergletschert war, und dass die Eismassen, welche über unser Land ihren Weg genommen, von hier nach dem Unterrhein hin fortflossen. Unsere nächste Aufgabe sei es, die Heimat der Geschiebe festzustellen. In einer weiteren Abhandlung soll die Gliederung des Diluviums zum Gegenstand der Untersuchung gemacht werden, und im Anschluss hieran gedenke ich meinen Ansichten über die diluvialen Höhen Hollands und des angrenzenden Hannovers eine eingehendere Begründung zu Teil werden zu lassen, als mir dies im Rahmen meiner letzten erschienenen Arbeit möglich war. Endlich soll der Frage nähergetreten werden, welches Alter wir unserm Diluvium beizumessen haben, und welche Stellung es zu den Glacialablagerungen des Ostens und des Nordens einnimmt.
In der vorliegenden Arbeit wird die naturräumliche Gliederung im Raum Bochum und Herne (mittleres Ruhrgebiet) vorgestellt. Hier treffen das Norddeutsche Tiefland mit der Emschertalung und dem lössüberprägten Westenhellweg sowie die Deutsche Mittelgebirgsschwelle in Form des Ruhrtals aufeinander und sorgen für ein von Natur aus abwechslungsreiches Relief mit unterschiedlichen Standortbedingungen. Der Artikel soll einen Beitrag für das Verständnis der ursprünglichen wie heutigen physisch-geographischen Verhältnisse im Gebiet leisten. Er vermittelt einen Überblick über Stadtgeographie, naturräumliche Gliederung, Geologie, Geomorphologie, Boden, Klima und Vegetation im Raum Bochum und Herne. Der Schwerpunkt liegt dabei auf der Darstellung der Oberflächenformen und der potentiellen natürlichen Vegetation.
Die Ergebnisse der Beobachtungen der meteorologischen Station zu Osnabrück in den Jahren 1891 und 1892 sind in Form von Tabellen und Diagrammen zusammengefasst. Bei den Ergebnissen handelt es sich um die Regenhöhe, die Temperatur, die relative Feuchtigkeit, der Dunstdruck, die Windrichtung und der Druck.
Keskinen, Helmi ; Virtanen, Annele ; Joutsensaari, Jorma ; Tsagkogeorgas, Georgios ; Duplissy, Jonathan ; Schobesberger, Siegfried ; Gysel, Martin ; Riccobono, Francesco ; Slowik, Jay G. ; Bianchi, Federico ; Yli-Juuti, Taina ; Lehtipalo, Katrianne ; Rondo, Linda ; Breitenlechner, Martin ; Kupc, Agnieszka ; Almeida, Joao ; Amorin, António ; Dunne, Eimear M. ; Downward, Andrew J. ; Ehrhart, Sebastian ; Franchin, Alessandro ; Kajos, Maija K. ; Kirkby, Jasper ; Kürten, Christoph Andreas ; Nieminen, Tuomo ; Makhmutov, Vladimir ; Mathot, Serge ; Miettinen, Pasi ; Onnela, Antti ; Petäjä, Tuukka ; Praplan, Arnaud Patrick ; Santos, Filipe Duarte ; Schallhart, Simon ; Sipilä, Mikko ; Stozhkov, Yuri ; Tomé, Antonio ; Vaattovaara, Petri ; Wimmer, Daniela ; Prévôt, André Stephan Henry ; Dommen, Josef ; Donahue, Neil McPherson ; Flagan, Richard C. ; Weingartner, Ernest ; Viisanen, Yrjö ; Riipinen, Ilona ; Hansel, Armin ; Curtius, Joachim ; Kulmala, Markku ; Worsnop, Douglas R. ; Baltensperger, Urs ; Wex, Heike ; Stratmann, Frank ; Laaksonen, Ari
Sulphuric acid, ammonia, amines, and oxidised organics play a crucial role in nanoparticle formation in the atmosphere. In this study, we investigate the composition of nucleated nanoparticles formed from these compounds in the CLOUD (Cosmics Leaving Outdoor Droplets) chamber experiments at CERN (Centre européen pour la recherche nucléaire). The investigation was carried out via analysis of the particle hygroscopicity, ethanol affinity, oxidation state, and ion composition. Hygroscopicity was studied by a hygroscopic tandem differential mobility analyser and a cloud condensation nuclei counter, ethanol affinity by an organic differential mobility analyser and particle oxidation level by a high-resolution time-of-flight aerosol mass spectrometer. The ion composition was studied by an atmospheric pressure interface time-of-flight mass spectrometer. The volume fraction of the organics in the particles during their growth from sizes of a few nanometers to tens of nanometers was derived from measured hygroscopicity assuming the Zdanovskii–Stokes–Robinson relationship, and compared to values gained from the spectrometers. The ZSR-relationship was also applied to obtain the measured ethanol affinities during the particle growth, which were used to derive the volume fractions of sulphuric acid and the other inorganics (e.g. ammonium salts). In the presence of sulphuric acid and ammonia, particles with a mobility diameter of 150 nm were chemically neutralised to ammonium sulphate. In the presence of oxidation products of pinanediol, the organic volume fraction of freshly nucleated particles increased from 0.4 to ~0.9, with an increase in diameter from 2 to 63 nm. Conversely, the sulphuric acid volume fraction decreased from 0.6 to 0.1 when the particle diameter increased from 2 to 50 nm. The results provide information on the composition of nucleated aerosol particles during their growth in the presence of various combinations of sulphuric acid, ammonia, dimethylamine and organic oxidation products.
Da bei den bis jetzt über die Umgebung von Osnabrück publizierten geologischen Karten bei ihrem kleinen Massstabe auf eine Wiedergabe der genaueren Details verzichtet werden musste und auch zum Teil wenigstens die durch dieselben gegebene Darstellung der Verbreitung der einzelnen Formationen sich als ungenau erwies, so sind wir schon seit längerer Zeit bemüht gewesen, Material zum Zwecke genauerer geognostischer Aufnahmen zusammenzubringen. Zunächst hatten wir unser Augenmerk darauf gerichtet, die Trias-Formation einer spezielleren Untersuchung zu unterziehen und die Verbreitung ihrer-einzelnen Gliedern auf Blättern der hannoverschen Generalstabskarte genauer zur Darstellung zu bringen.
Hobe, Marc von ; Bekki, Slimane ; Borrmann, Stephan ; Cairo, Francesco ; D'Amato, Francesco ; Di Donfrancesco, Guido ; Dörnbrack, Andreas ; Ebersoldt, Andreas ; Ebert, Martin ; Emde, Claudia ; Engel, Ines ; Ern, Manfred ; Frey, Wiebke ; Genco, Silvia ; Griessbach, Sabine ; Grooß, Jens-Uwe ; Gulde, Thomas ; Günther, Gebhard ; Hösen, Elisabeth ; Hoffmann, Lars ; Homonnai, Viktoria ; Hoyle, Christopher Robert ; Isaksen, Ivar S.A. ; Jackson, David R. ; Jánosi, Imre M. ; Jones, Rod L. ; Kandler, Konrad ; Kalicinsky, Christoph ; Keil, Andrea ; Khaykin, Sergey M. ; Khosrawi, Farahnaz ; Kivi, Rigel ; Kuttippurath, Jayan ; Laube, Johannes Christian ; Lefèvre, Franck ; Lehmann, Ralph ; Ludmann, Sabrina ; Luo, Beiping P. ; Marchand, Marion ; Meyer, Jessica ; Mitev, Valentin ; Molleker, Sergej ; Müller, Rolf ; Oelhaf, Hermann ; Olschewski, Friedhelm ; Orsolini, Yvan ; Peter, Thomas ; Pfeilsticker, Klaus ; Piesch, Christof ; Pitts, Michael C. ; Poole, Lamont R. ; Pope, Francis D. ; Ravegnani, Fabrizio ; Rex, Markus ; Riese, Martin ; Röckmann, Thomas ; Rognerud, Bjørg ; Roiger, Anke ; Rolf, Christian ; Santee, Michelle L. ; Scheibe, Monika ; Schiller, Cornelius ; Schlager, Hans ; Siciliani de Cumis, Matteo ; Sitnikov, Nikolay ; Søvde, Ole Amund ; Spang, Reinhold ; Spelten, Nicole ; Stordal, Frode ; Sumińska-Ebersoldt, Olga ; Viciani, Silvia ; Volk, C.-Michael ; vom Scheidt, Marcel ; Ulanovski, Alexey ; Gathen, Peter von der ; Walker, Kaley A. ; Wegner, Tobias ; Weigel, Ralf ; Weinbruch, Stephan ; Wetzel, Gerald ; Wienhold, Franck G. ; Wohltmann, Ingo ; Woiwode, Wolfgang ; Young, Isla A. K. ; Yushkov, Vladimir ; Zobrist, Bernhard ; Stroh, Fred
The international research project RECONCILE has addressed central questions regarding polar ozone depletion, with the objective to quantify some of the most relevant yet still uncertain physical and chemical processes and thereby improve prognostic modelling capabilities to realistically predict the response of the ozone layer to climate change. This overview paper outlines the scope and the general approach of RECONCILE, and it provides a summary of observations and modelling in 2010 and 2011 that have generated an in many respects unprecedented dataset to study processes in the Arctic winter stratosphere. Principally, it summarises important outcomes of RECONCILE including (i) better constraints and enhanced consistency on the set of parameters governing catalytic ozone destruction cycles, (ii) a better understanding of the role of cold binary aerosols in heterogeneous chlorine activation, (iii) an improved scheme of polar stratospheric cloud (PSC) processes that includes heterogeneous nucleation of nitric acid trihydrate (NAT) and ice on non-volatile background aerosol leading to better model parameterisations with respect to denitrification, and (iv) long transient simulations with a chemistry-climate model (CCM) updated based on the results of RECONCILE that better reproduce past ozone trends in Antarctica and are deemed to produce more reliable predictions of future ozone trends. The process studies and the global simulations conducted in RECONCILE show that in the Arctic, ozone depletion uncertainties in the chemical and microphysical processes are now clearly smaller than the sensitivity to dynamic variability.
Hall, Brad D. ; Engel, Andreas ; Mühle, Jens ; Elkins, James William ; Artuso, Florinda ; Atlas, Elliot L. ; Aydin, Murat ; Blake, Donald R. ; Brunke, Ernst-Günther ; Chiavarini, Salvatore ; Fraser, Paul J. ; Happell, James D. ; Krummel, Paul B. ; Levin, Ingeborg ; Loewenstein, Max ; Maione, Michela ; Montzka, Stephen A. ; O'Doherty, Simon ; Reimann, Stefan ; Rhoderick, George J. ; Saltzman, Eric S. ; Scheel, Hans-Eckhart ; Steele, L. Paul ; Vollmer, Martin K. ; Weiss, Ray F. ; Worthy, Douglas E. ; Yokouchi, Yoko
The International Halocarbons in Air Comparison Experiment (IHALACE) was conducted to document relationships between calibration scales among various laboratories that measure atmospheric greenhouse and ozone depleting gases. Six stainless steel cylinders containing natural and modified natural air samples were circulated among 19 laboratories. Results from this experiment reveal relatively good agreement among commonly used calibration scales for a number of trace gases present in the unpolluted atmosphere at pmol mol−1 (parts per trillion) levels, such as chlorofluorocarbons (CFCs), hydrochlorofluorocarbons (HCFCs), and hydrofluorocarbons (HFCs). Some scale relationships were found to be consistent with those derived from bi-lateral experiments or from analysis of atmospheric data, while others revealed discrepancies. The transfer of calibration scales among laboratories was found to be problematic in many cases, meaning that measurements tied to a common scale may not, in fact, be compatible. These results reveal substantial improvements in calibration over previous comparisons. However there is room for improvement in communication and coordination of calibration activities with respect to the measurement of halogenated and related trace gases.
Nölscher, Anke Christine ; Bourtsoukidis, Efstratios ; Bonn, Boris ; Kesselmeier, Jürgen ; Lelieveld, Johannes ; Williams, Jonathan
Numerous reactive volatile organic compounds (VOCs) are emitted into the atmosphere by vegetation. Most biogenic VOCs are highly reactive towards the atmosphere's most important oxidant, the hydroxyl (OH) radical. One way to investigate the chemical interplay between biosphere and atmosphere is through the measurement of total OH reactivity, the total loss rate of OH radicals. This study presents the first determination of total OH reactivity emission rates (measurements via the comparative reactivity method) based on a branch cuvette enclosure system mounted on a Norway spruce (Picea abies) throughout spring, summer and autumn 2011. In parallel VOC emission rates were monitored by a second proton-transfer-reaction mass spectrometer (PTR-MS), and total ozone (O3) loss rates were obtained inside the cuvette. Total OH reactivity emission rates were in general temperature and light dependent, showing strong diel cycles with highest values during daytime. Monoterpene emissions contributed most, accounting for 56–69% of the measured total OH reactivity flux in spring and early summer. However, during late summer and autumn the monoterpene contribution decreased to 11–16%. At this time, a large missing fraction of the total OH reactivity emission rate (70–84%) was found when compared to the VOC budget measured by PTR-MS. Total OH reactivity and missing total OH reactivity emission rates reached maximum values in late summer corresponding to the period of highest temperature. Total O3 loss rates within the closed cuvette showed similar diel profiles and comparable seasonality to the total OH reactivity fluxes.
Total OH reactivity fluxes were also compared to emissions from needle storage pools predicted by a temperature-only-dependent algorithm. Deviations of total OH reactivity fluxes from the temperature-only-dependent emission algorithm were observed for occasions of mechanical and heat stress. While for mechanical stress, induced by strong wind, measured VOCs could explain total OH reactivity emissions, during heat stress they could not. The temperature-driven algorithm matched the diel variation of total OH reactivity emission rates much better in spring than in summer, indicating a different production and emission scheme for summer and early autumn. During these times, unmeasured and possibly unknown primary biogenic emissions contributed significantly to the observed total OH reactivity flux.
Buchbesprechungen
(1996)
Besprochen werden die beiden folgenden Werke:
(1) Handbuch der Bodenkunde - Grundwerk. Von H. P. Blume , P. Felix-Henningsen, W.R. Fischer, H.-G. Frede, R. Horn u. K. Stahr.
(2) Thienemann, Johannes: Rossitten - drei Jahrzehnte auf der Kurischen Nehrung. Reprint der Ausgabe Melsungen, Neumann-Neudamm von 1930 (3.Aufl.).
has been demonstrated in climate models that both the Indian and East Asian summer monsoons (ISM and EASM) are strengthened by the uplift of the entire Asian orography or Tibetan Plateau (TP) (i.e. bulk mountain uplift). Such an effect is widely perceived as the major mechanism contributing to the evolution of Asian summer monsoons in the Neogene. However, geological evidence suggests more diachronous growth of the Asian orography (i.e. regional mountain uplift) than bulk mountain uplift. This demands a re-evaluation of the relation between mountain uplift and the Asian monsoon in the geological periods. In this study, sensitivity experiments considering the diachronous growth of different parts of the Asian orography are performed using the regional climate model COSMO-CLM to investigate their effects on the Asian summer monsoons. The results show that, different from the bulk mountain uplift, the regional mountain uplift can lead to an asynchronous development of the ISM and EASM. While the ISM is primarily intensified by the thermal insulation (mechanical blocking) effect of the southern TP (Zagros Mountains), the EASM is mainly enhanced by the surface sensible heating of the central, northern and eastern TP. Such elevated surface heating can induce a low-level cyclonic anomaly around the TP that reduces the ISM by suppressing the lower tropospheric monsoon vorticity, but promotes the EASM by strengthening the warm advection from the south of the TP that sustains the monsoon convection. Our findings provide new insights to the evolution of the Asian summer monsoons and their interaction with the tectonic changes in the Neogene.
Spatial interpolation of rain gauge data is important in forcing of hydrological simulations or evaluation of weather predictions, for example. This paper investigates the application of statistical distance, like one minus common variance of observation time series, between data sites instead of geographical distance in interpolation. Here, as a typical representative of interpolation methods the inverse distance weighting interpolation is applied and the test data is daily precipitation observed in Austria. Choosing statistical distance instead of geographical distance in interpolation of available coarse network observations to sites of a denser network, which is not reporting for the interpolation date, yields more robust interpolation results. The most distinct performance enhancement is in or close to mountainous terrain. Therefore, application of statistical distance in the inverse distance weighting interpolation or in similar methods can parsimoniously densify the currently available observation network. Additionally, the success further motivates search for conceptual rain-orography interaction models as components of spatial rain interpolation algorithms in mountainous terrain.
Spatial interpolation of rain gauge data is important in forcing of hydrological simulations or evaluation of weather predictions, for example. The spatial density of available data sites is often changing with time. This paper investigates the application of statistical distance, like one minus common variance of time series, between data sites instead of geographical distance in interpolation. Here, as a typical representative of interpolation methods the inverse distance weighting interpolation is applied and the test data is daily precipitation observed in Austria. Choosing statistical distance instead of geographical distance in interpolation of an actually available coarse observation network yields more robust interpolation results at sites of a denser network with actually lacking observations. The performance enhancement is in or close to mountainous terrain. This has the potential to parsimoniously densify the currently available observation network. Additionally, the success further motivates search for conceptual rain-orography interaction models as components of spatial rain interpolation algorithms in mountainous terrain.
In this study, two different methods were applied to derive daily and monthly sunshine duration based on high-resolution satellite products provided by the European Organisation for the Exploitation of Meteorological Satellites (EUMETSAT) Satellite Application Facility on Climate Monitoring using data from Meteosat Second Generation (MSG) SEVIRI (Spinning Enhanced Visible and Infrared Imager). The satellite products were either hourly cloud type or hourly surface incoming direct radiation. The satellite sunshine duration estimates were not found to be significantly different using the native 15-minute temporal resolution of SEVIRI. The satellite-based sunshine duration products give additional spatial information over the European continent compared with equivalent in situ-based products. An evaluation of the satellite sunshine duration by product intercomparison and against station measurements was carried out to determine their accuracy. The satellite data were found to be within ±1 h/day compared to high-quality Baseline Surface Radiation Network or surface synoptic observations (SYNOP) station measurements. The satellite-based products differ more over the oceans than over land, mainly because of the treatment of fractional clouds in the cloud type-based sunshine duration product. This paper presents the methods used to derive the satellite sunshine duration products and the performance of the different retrievals. The main benefits and disadvantages compared to station-based products are also discussed.