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Two-center level diagrams for the neutron orbitals in the scattering of 16O on 25Mg and of 17O on 24Mg are calculated by using a deformed potential for 24,25Mg. Possible consequences of the nuclear Landau-Zener mechanism, namely the promotion of nucleons at avoided level crossings, and of the rotational coupling between crossing molecular single-particle orbitals are studied for inelastic excitation and neutron transfer. The important excitation and transfer processes, which are enhanced by the promotion process and the rotational coupling, are presented. NUCLEAR REACTIONS Heavy ion scattering, theory of nucleon transfer, molecular wave functions, asymmetric two center shell model, single particle excitation, deformed nuclei.
In heavy ion collisions, the molecular single-particle motion may cause specific structures in the energy dependence of the cross sections which arise by the promotion of nucleons at level crossings according to the Landau-Zener excitation mechanism. In order to examine this effect in asymmetric heavy ion collisions, we have calculated level diagrams of the two-center shell model for the target projectile combinations 13C + 16O and 12C + 17O and analyzed with respect to inelastic excitation and neutron transfer. We select certain reactions as possible candidates for showing enhanced cross sections for nucleon excitation and transfer due to real and avoided level crossings near the Fermi level.
With a schematic model for the nuclear matter we give a unified treatment of the real and imaginary parts of the elastic O16-O16 scattering potential. The model connects the parameters of the potential with the density and binding properties of the O16-O16 system and reproduces the structure of the excitation function quite well. It is shown that the nuclear compressibility can be obtained from the scattering data, and in the case of the S32 compound system there results an effective compressibility (finite quenching of the nuclei) of about 200 MeV.
For cold (neutronless) fission we consider an analytical model of quantum tunneling with dissipation through a barrier U(q) evaluated with a M3Y nucleon-nucleon force. We calculate the tunneling spectrum, i.e., the fission rate as a function of the total kinetic energy of the fragments. The theoretical results are compared with the experimental data obtained for the fine structure of two cold fission modes of 252Cf: 148Ba+104Mo and 146Ba+106Mo. Taking into account the dissipative coupling of the potential function U(q) and of the momentum p with all the other neglected coordinates, we obtain a remarkable agreement with the experimental data. We conclude that the cold fission process is a spontaneous decay with a spectrum determined by the shape of the barrier and an amplitude depending on the strength of the dissipative coupling.
The molecular particle-core model is applied to the scattering of 13C on 13C. The model divides the 13C+ 13C system into two 12C cores and two valence neutrons. The valence neutrons are described with molecular eigenfunctions of the symmetric two-center shell model. Coupled channel calculations are carried out for the inelastic single and mutual excitation of the first (1/2+ state of 13C and the neutron transfer to the 12C+14C system. The results reproduce the experimental data. The analysis of the S matrix shows that the gross structure of the transfer excitation function is related to resonances in the relative motion of the elastic and transfer channels.
The inelastic excitation of the (1/2)+ (871 keV) state of 17O in the reaction of 13C on 17O is described by a time-dependent quantum mechanical model with two diabatic states and a classical treatment of the radial relative motion. The structures in the angle-integrated cross section are interpreted as caused by the barriers of the angular momentum-dependent potentials. The transition strength is enhanced by the Landau-Zener effect between the levels considered.
Determination of the effective 12C + 12C potential from the sub-Coulomb single-particle resonances
(1974)
The sub-Coulomb resonances observed in the total reaction yield of the 12C + 12C system at 4.9, 5.6, and 6.2 MeV are explained as single-particle resonances. The "true" effective 12C + 12C potential is determined directly as the real potential which reproduces best the position and the spacing of the observed sub-Coulomb resonances. This potential is found from a parametrization of the two limiting adiabatic and sudden potentials.