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Hoyle, Christopher Robert ; Fuchs, Claudia ; Järvinen, Emma ; Saathoff, Harald ; Dias, Antonio ; El Haddad, Imad ; Gysel, Martin ; Coburn, Sean C. ; Tröstl, Jasmin ; Bernhammer, Anne-Kathrin ; Bianchi, Federico ; Breitenlechner, Martin ; Corbin, Joel C. ; Craven, Jill ; Donahue, Neil McPherson ; Duplissy, Jonathan ; Ehrhart, Sebastian ; Frege, Carla ; Gordon, Hamish ; Höppel, Niko Florian ; Heinritzi, Martin ; Kristensen, Thomas Bjerring ; Molteni, Ugo ; Nichman, Leonid ; Pinterich, Tamara ; Prévôt, André Stephan Henry ; Simon, Mario ; Slowik, Jay G. ; Steiner, Gerhard ; Tomé, Antonio ; Vogel, Alexander L. ; Volkamer, Rainer ; Wagner, Andrea Christine ; Wagner, Robert ; Wexler, Anthony S. ; Williamson, Christina ; Winkler, Paul M. ; Yan, Chao ; Amorim, Antonio ; Dommen, Josef ; Curtius, Joachim ; Gallagher, Martin William ; Flagan, Richard C. ; Hansel, Armin ; Kirkby, Jasper ; Kulmala, Markku ; Möhler, Ottmar ; Stratmann, Frank ; Worsnop, Douglas R. ; Baltensperger, Urs
The growth of aerosol due to the aqueous phase oxidation of sulfur dioxide by ozone was measured in laboratory-generated clouds created in the Cosmics Leaving OUtdoor Droplets (CLOUD) chamber at the European Organization for Nuclear Research (CERN). Experiments were performed at 10 and −10 °C, on acidic (sulfuric acid) and on partially to fully neutralised (ammonium sulfate) seed aerosol. Clouds were generated by performing an adiabatic expansion – pressurising the chamber to 220 hPa above atmospheric pressure, and then rapidly releasing the excess pressure, resulting in a cooling, condensation of water on the aerosol and a cloud lifetime of approximately 6 min. A model was developed to compare the observed aerosol growth with that predicted using oxidation rate constants previously measured in bulk solutions. The model captured the measured aerosol growth very well for experiments performed at 10 and −10 °C, indicating that, in contrast to some previous studies, the oxidation rates of SO2 in a dispersed aqueous system can be well represented by using accepted rate constants, based on bulk measurements. To the best of our knowledge, these are the first laboratory-based measurements of aqueous phase oxidation in a dispersed, super-cooled population of droplets. The measurements are therefore important in confirming that the extrapolation of currently accepted reaction rate constants to temperatures below 0 °C is correct.
Hoyle, Christopher Robert ; Fuchs, Claudia ; Järvinen, Emma ; Saathoff, Harald ; Dias, Antonio ; El Haddad, Imad ; Gysel, Martin ; Coburn, Sean C. ; Tröstl, Jasmin ; Bernhammer, Anne-Kathrin ; Bianchi, Federico ; Breitenlechner, Martin ; Corbin, Joel C. ; Craven, Jill ; Donahue, Neil McPherson ; Duplissy, Jonathan ; Ehrhart, Sebastian ; Frege, Carla ; Gordon, Hamish ; Höppel, Niko Florian ; Heinritzi, Martin ; Kristensen, Thomas Bjerring ; Molteni, Ugo ; Nichman, Leonid ; Pinterich, Tamara ; Prévôt, André Stephan Henry ; Simon, Mario ; Slowik, Jay G. ; Steiner, Gerhard ; Tomé, Antonio ; Vogel, Alexander L. ; Volkamer, Rainer ; Wagner, Andrea Christine ; Wagner, Robert ; Wexler, Anthony S. ; Williamson, Christina ; Winkler, Paul M. ; Yan, Chao ; Amorim, Antonio ; Dommen, Josef ; Curtius, Joachim ; Gallagher, Martin William ; Flagan, Richard C. ; Hansel, Armin ; Kirkby, Jasper ; Kulmala, Markku ; Möhler, Ottmar ; Stratmann, Frank ; Worsnop, Douglas R. ; Baltensperger, Urs
The growth of aerosol due to the aqueous phase oxidation of sulfur dioxide by ozone was measured in laboratory-generated clouds created in the Cosmics Leaving OUtdoor Droplets (CLOUD) chamber at the European Organization for Nuclear Research (CERN). Experiments were performed at 10 and −10 °C, on acidic (sulfuric acid) and on partially to fully neutralised (ammonium sulfate) seed aerosol. Clouds were generated by performing an adiabatic expansion – pressurising the chamber to 220 hPa above atmospheric pressure, and then rapidly releasing the excess pressure, resulting in a cooling, condensation of water on the aerosol and a cloud lifetime of approximately 6 min. A model was developed to compare the observed aerosol growth with that predicted using oxidation rate constants previously measured in bulk solutions. The model captured the measured aerosol growth very well for experiments performed at 10 and −10 °C, indicating that, in contrast to some previous studies, the oxidation rates of SO2 in a dispersed aqueous system can be well represented by using accepted rate constants, based on bulk measurements. To the best of our knowledge, these are the first laboratory-based measurements of aqueous phase oxidation in a dispersed, super-cooled population of droplets. The measurements are therefore important in confirming that the extrapolation of currently accepted reaction rate constants to temperatures below 0 °C is correct.
Kirkby, Jasper ; Duplissy, Jonathan ; Sengupta, Kamalika ; Frege, Carla ; Gordon, Hamish ; Williamson, Christina ; Heinritzi, Martin ; Simon, Mario ; Yan, Chao ; Almeida, Joao ; Tröstl, Jasmin ; Nieminen, Tuomo ; Ortega, Ismael K. ; Wagner, Robert ; Adamov, Alexey ; Amorim, Antonio ; Bernhammer, Anne-Kathrin ; Bianchi, Federico ; Breitenlechner, Martin ; Brilke, Sophia ; Chen, Xuemeng ; Craven, Jill ; Dias, Antonio ; Ehrhart, Sebastian ; Flagan, Richard C. ; Franchin, Alessandro ; Fuchs, Claudia ; Guida, Roberto ; Hakala, Jani ; Hoyle, Christopher Robert ; Jokinen, Tuija ; Junninen, Heikki ; Kangasluoma, Juha ; Kim, Jaeseok ; Krapf, Manuel ; Kürten, Christoph Andreas ; Laaksonen, Ari ; Lehtipalo, Katrianne ; Makhmutov, Vladimir ; Mathot, Serge ; Molteni, Ugo ; Onnela, Antti ; Peräkylä, Otso ; Piel, Felix ; Petäjä, Tuukka ; Praplan, Arnaud Patrick ; Pringle, Kirsty ; Rap, Alexandru ; Richards, Nigel A. D. ; Riipinen, Ilona ; Rissanen, Matti P. ; Rondo, Linda ; Sarnela, Nina ; Schobesberger, Siegfried ; Scott, Catherine E. ; Seinfeld, John H. ; Sipilä, Mikko ; Steiner, Gerhard ; Stozhkov, Yuri ; Stratmann, Frank ; Tomé, Antonio ; Virtanen, Annele ; Vogel, Alexander L. ; Wagner, Andrea Christine ; Wagner, Paul E. ; Weingartner, Ernest ; Wimmer, Daniela ; Winkler, Paul M. ; Ye, Penglin ; Zhang, Xuan ; Hansel, Armin ; Dommen, Josef ; Donahue, Neil McPherson ; Worsnop, Douglas R. ; Baltensperger, Urs ; Kulmala, Markku ; Carslaw, Kenneth S. ; Curtius, Joachim
Atmospheric aerosols and their effect on clouds are thought to be important for anthropogenic radiative forcing of the climate, yet remain poorly understood1. Globally, around half of cloud condensation nuclei originate from nucleation of atmospheric vapours2. It is thought that sulfuric acid is essential to initiate most particle formation in the atmosphere3,4, and that ions have a relatively minor role5. Some laboratory studies, however, have reported organic particle formation without the intentional addition of sulfuric acid, although contamination could not be excluded6,7. Here we present evidence for the formation of aerosol particles from highly oxidized biogenic vapours in the absence of sulfuric acid in a large chamber under atmospheric conditions. The highly oxygenated molecules (HOMs) are produced by ozonolysis of α-pinene. We find that ions from Galactic cosmic rays increase the nucleation rate by one to two orders of magnitude compared with neutral nucleation. Our experimental findings are supported by quantum chemical calculations of the cluster binding energies of representative HOMs. Ion-induced nucleation of pure organic particles constitutes a potentially widespread source of aerosol particles in terrestrial environments with low sulfuric acid pollution.
Harrison, Sandy P. ; Villegas-Diaz, Roberto ; Cruz-Silva, Esmeralda ; Gallagher, Daniel ; Kesner, David ; Lincoln, Paul ; Shen, Yicheng ; Sweeney, Luke ; Colombaroli, Daniele ; Ali, Adam ; Barhoumi, Chéïma ; Bergeron, Yves ; Blyakharchuk, Tatiana ; Bobek, Přemysl ; Bradshaw, Richard ; Clear, Jennifer L. ; Czerwiński, Sambor ; Daniau, Anne-Laure ; Dodson, John ; Edwards, Kevin J. ; Edwards, Mary E. ; Feurdean, Angelica ; Foster, David ; Gajewski, Konrad ; Gałka, Mariusz ; Garneau, Michelle ; Giesecke, Thomas ; Gil Romera, Graciela ; Girardin, Martin P. ; Höfer, Dana ; Huang, Kangyou ; Inoue, Jun ; Jamrichová, Eva ; Jasiunas, Nauris ; Jiang, Wenying ; Jiménez-Moreno, Gonzalo ; Karpińska-Kołaczek, Monika ; Kołaczek, Piotr ; Kuosmanen, Niina ; Lamentowicz, Mariusz ; Lavoie, Martin ; Li, Fang ; Li, Jianyong ; Lisitsyna, Olga ; López-Sáez, José Antonio ; Luelmo-Lautenschlaeger, María de los Reyes ; Magnan, Gabriel ; Magyari, Eniko Katalin ; Maksims, Alekss ; Marcisz, Katarzyna ; Marinova, Elena ; Marlon, Jenn ; Mensing, Scott ; Miroslaw-Grabowska, Joanna ; Oswald, Wyatt ; Pérez-Dı́az, Sebastián ; Pérez-Obiol, Ramón ; Piilo, Sanna ; Poska, Anneli ; Qin, Xiaoguang ; Remy, Cécile ; Richard, Pierre J. H. ; Salonen, Sakari ; Sasaki, Naoko ; Schneider, Heike ; Shotyk, William ; Stančikaitė, Migle ; Šteinberga, Dace ; Stivriņš, Normunds ; Takahara, Hikaru ; Tan, Zhihai ; Trasune, Liva ; Umbanhowar, Charles E. ; Väliranta, Minna ; Vassiljev, Jüri ; Xiao, Xiayun ; Xu, Qinghai ; Xu, Xin ; Zawisza, Edyta ; Zhao, Yan ; Zhou, Zheng ; Paillard, Jordan
Sedimentary charcoal records are widely used to reconstruct regional changes in fire regimes through time in the geological past. Existing global compilations are not geographically comprehensive and do not provide consistent metadata for all sites. Furthermore, the age models provided for these records are not harmonised and many are based on older calibrations of the radiocarbon ages. These issues limit the use of existing compilations for research into past fire regimes. Here, we present an expanded database of charcoal records, accompanied by new age models based on recalibration of radiocarbon ages using IntCal20 and Bayesian age-modelling software. We document the structure and contents of the database, the construction of the age models, and the quality control measures applied. We also record the expansion of geographical coverage relative to previous charcoal compilations and the expansion of metadata that can be used to inform analyses. This first version of the Reading Palaeofire Database contains 1676 records (entities) from 1480 sites worldwide. The database (RPDv1b – Harrison et al., 2021) is available at https://doi.org/10.17864/1947.000345.
Recent expeditions (NANHAI 2014, DONGSHA 2014 and ZHONGSHA 2015) conducted in deep waters of the South China Sea obtained interesting material of various spider crabs (Majoidea) including several new records for the area, and two new species of epialtids of the genera Oxypleurodon Miers, 1885 and Stegopleurodon Richer de Forges & Ng, 2009. Two poorly known species, previously only known from their types, Rochinia strangeri Serène & Lohavanijaya, 1973 and R. kagoshimensis (Rathbun, 1932) comb. nov., are redescribed, refigured, and their taxonomy discussed.
Öztürk, Fatma Cagla ; Akkuş, Baki ; Atanasov, Dinko ; Beyer, Heinrich F. ; Bosch, Fritz ; Boutin, David ; Brandau, Carsten ; Bühler, Paul ; Çakirli Mutlu, Rabia Burcu ; Chen, Ruijiu ; Chen, Weidong ; Chen, Xiangcheng ; Dillmann, Iris ; Dimopoulou, Christina ; Enders, Wolfgang ; Essel, Hans G. ; Faestermann, Thomas ; Forstner, Oliver ; Gao, Bing-Shui ; Geissel, Hans ; Gernhäuser, Roman ; Grisenti, Robert Evaristo ; Gumberidze, Alexandre ; Hagmann, Siegbert ; Heftrich, Tanja ; Heil, Michael ; Herdrich, Marc Oliver ; Hillenbrand, Pierre-Michel ; Izumikawa, Takuji ; Kienle, Paul ; Klaushofer, Christoph ; Kleffner, Carl-Michael ; Kozhuharov, Christophor ; Knöbel, Ronja ; Kovalenko, Oleksandr ; Kreim, Susanne ; Kühl, Thomas ; Lederer-Woods, Claudia ; Lestinsky, Michael ; Litvinov, Sergey A. ; Litvinov, Yuri A. ; Liu, Zhong ; Ma, Xinwen ; Maier, Ludwig W. ; Mei, Bo ; Miura, Hiroshi ; Mukha, Ivan ; Najafi, Mohammad Ali ; Nagae, Daisuke ; Nishimura, Takuro ; Nociforo, Chiara ; Nolden, Fritz ; Ohtsubo, Takashi ; Öktem, Yeşim ; Omika, Shunichiro ; Ozawa, Akira ; Petridis, Nikolaos ; Piotrowski, Jeremi ; Reifarth, René ; Roßbach, Jörg ; Sánchez Alarcón, Rodolfo Marcelo ; Sanjari, Mohammad Shahab ; Scheidenberger, Christoph ; Sidhu, Ragandeep Singh ; Simon, Haik ; Spillmann, Uwe ; Steck, Markus ; Stöhlker, Thomas ; Sun, Baohua ; Susam, Lidya Amon ; Suzaki, Fumi ; Suzuki, Takeshi ; Torilov, Sergey Yu. ; Trageser, Christian ; Trassinelli, Martino ; Trotsenko, Sergiy ; Tu, Xiaolin ; Walker, Philip M. ; Wang, M. ; Weber, Günter ; Weick, Helmut ; Winckler, Nicolas ; Winters, Danyal Ferdinant Alexander ; Woods, Philip John ; Yamaguchi, Takayuki ; Xu, X.D. ; Yan, X.L. ; Yang, Jiancheng ; Yuan, You-Jin ; Zhang, Yuhu ; Zhou, Xiaohong
An experiment addressing electron capture (EC) decay of hydrogen-like 142Pm60+ions has been conducted at the experimental storage ring (ESR) at GSI. The decay appears to be purely exponential and no modulations were observed. Decay times for about 9000 individual EC decays have been measured by applying the single-ion decay spectroscopy method. Both visually and automatically analysed data can be described by a single exponential decay with decay constants of 0.0126(7)s−1 for automatic analysis and 0.0141(7)s−1 for manual analysis. If a modulation superimposed on the exponential decay curve is assumed, the best fit gives a modulation amplitude of merely 0.019(15), which is compatible with zero and by 4.9 standard deviations smaller than in the original observation which had an amplitude of 0.23(4).