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The subject of this thesis is the experimental investigation of the neutron-capture cross sections of the neutron-rich, short-lived boron isotopes 13B and 14B, as they are thought to influence the rapid neutron-capture process (r process) nucleosynthesis in a neutrino-driven wind scenario.
The 13;14B(n,g)14;15B reactions were studied in inverse kinematics via Coulomb dissociation at the LAND/R3B setup (Reactions with Relativistic Radioactive Beams). A radioactive beam of 14;15B was produced via in-flight fragmentation and directed onto a lead-target at about 500 AMeV. The neutron breakup of the projectile within the electromagnetic field of the target nucleus was investigated in a kinematically complete measurement. All outgoing reaction products were detected and analyzed in order to reconstruct the excitation energy.
The differential Coulomb dissociation cross sections as a function of the excitation energy were obtained and first experimental constraints on the photoabsorption and the neutron-capture cross sections were deduced. The results were compared to theoretical approximations of the cross sections in question. The Coulomb dissociation cross section of 15B into 14B(g.s.) + n was determined to be s(15B;14B(g:s:)+n) CD = 81(8stat)(10syst) mb ; while the Coulomb dissociation cross section of 14B into a neutron and 13B in its ground state was found to be s(14B;13B(g:s:)+n) CD = 281(25stat)(43syst) mb: Furthermore, new information on the nuclear structure of 14B were achieved, as the spectral shape of the differential Coulomb dissociation cross section indicates a halolike structure of the nucleus.
Additionally, the Coulomb dissociation of 11Be was investigated and compared to previous measurements in order to verify the present analysis. The corresponding Coulomb dissociation cross section of 11Be into 10Be(g.s.) + n was found to be 450(40stat)(54syst ) mb, which is in good agreement with the results of Palit et al.
Mingrone, Federica ; Massimi, Cristian ; Vannini, Gianni ; Altstadt, Sebastian ; Andrzejewski, Józef ; Audouin, Ludmila ; Barbagallo, Massimo ; Bécares, Vicente ; Bečvář, František ; Belloni, Fabio ; Berthoumieux, Eric ; Billowes, Jonathan ; Bosnar, Damir ; Brugger, Markus ; Calviani, Marco ; Calviño Tavares, Francisco ; Cano-Ott, Daniel ; Carrapiço, Carlos ; Cerutti, Francesco ; Chiaveri, Enrico ; Chin, Mary ; Colonna, Nicola ; Cortés Rossell, Guillem Pere ; Cortés-Giraldo, Miguel Antonio ; Diakaki, Maria ; Domingo-Pardo, César ; Durán, Ignacio ; Dressler, Rugard ; Eleftheriadis, Christos ; Ferrari, Alfredo ; Fraval, Kevin ; Ganesan, Srinivasan ; García Ríos, Aczel Regino ; Giubrone, Giuseppe ; Gonçalves, Isabel Maria Ferro ; González Romero, Enrique ; Griesmayer, Erich ; Guerrero Sánchez, Carlos ; Gunsing, Frank ; Hernández Prieto, Álvaro ; Jenkins, David ; Jericha, Erwin ; Kadi, Yacine ; Käppeler, Franz ; Karadimos, Dimitri ; Kivel, Nikolay ; Koehler, Paul Edward ; Krtička, Milan ; Kroll, Jiří ; Lampoudis, Christos ; Langer, Christoph ; Leal Cidoncha, Esther ; Lederer, Claudia ; Leeb, Helmut ; Leong, Lou Sai ; Losito, Roberto ; Mallick, Amod Kishore ; Manousos, Athanasios ; Marganiec, Justyna ; Martínez, Trinitario ; Mastinu, Pierfrancesco ; Mastromarco, Mario ; Mendoza Cembranos, Emilio ; Mengoni, Alberto ; Milazzo, Paolo Maria ; Mirea, Mihail ; Mondalaers, Willy ; Paradela Dobarro, Carlos ; Pavlik, Andreas ; Perkowski, Jarosław ; Plompen, Arjan J. M. ; Praena, Javier ; Quesada Molina, José Manuel ; Rauscher, Thomas ; Reifarth, René ; Riego Pérez, Albert ; Robles, Marisol S. ; Rubbia, Carlo ; Sabaté Gilarte, Marta ; Sarmento, Raul ; Saxena, Alok ; Schillebeeckx, Peter ; Schmidt, Sebastian ; Schumann, Dorothea ; Tagliente, Giuseppe ; Taı́n Enríquez, José Luis ; Tarrío Vilas, Diego ; Tassan-Got, Laurent ; Tsinganis, Andrea ; Valenta, Stanislav ; Variale, Vincenzo ; Vaz, Pedro ; Ventura, Alberto ; Vermeulen, Mark J. ; Vlachoudis, Vasilis ; Vlastou, Rosa ; Wallner, Anton ; Ware, Timothy ; Weigand, Mario ; Weiß, Christina ; Wright, Tobias ; Žugec, Petar
The radiative capture cross section of 238U is very important for the developing of new reactor technologies and the safety of existing ones. Here the preliminary results of the 238U(n,γ) cross section measurement performed at n_TOF with C6D6 scintillation detectors are presented, paying particular attention to data reduction and background subtraction.
We explore the parameter space of the two-flavor thermal quark–meson model and its Polyakov loop-extended version under the influence of a constant external magnetic field B. We investigate the behavior of the pseudo critical temperature for chiral symmetry breaking taking into account the likely dependence of two parameters on the magnetic field: the Yukawa quark–meson coupling and the parameter T0 of the Polyakov loop potential. Under the constraints that magnetic catalysis is realized at zero temperature and the chiral transition at B=0 is a crossover, we find that the quark–meson model leads to thermal magnetic catalysis for the whole allowed parameter space, in contrast to the present picture stemming from lattice QCD.
The ab-initio molecular dynamics framework has been the cornerstone of computational solid state physics in the last few decades. Although it is already a mature field it is still rapidly developing to accommodate the growth in solid state research as well as to efficiently utilize the increase in computing power. Starting from the first principles, the ab-initio molecular dynamics provides essential information about structural and electronic properties of matter under various external conditions. In this thesis we use the ab-initio molecular dynamics to study the behavior of BaFe2As2 and CaFe2As2 under the application of external pressure. BaFe2As2 and CaFe2As2 belong to the family of iron based superconductors which are a novel and promising superconducting materials. The application of pressure is one of two key methods by which electronic and structural properties of iron based superconductors can be modified, the other one being doping (or chemical pressure). In particular, it has been noted that pressure conditions have an important effect, but their exact role is not fully understood. To better understand the effect of different pressure conditions we have performed a series of ab-initio simulations of pressure application. In order to apply the pressure with arbitrary stress tensor we have developed a method based on the Fast Inertial Relaxation Engine, whereby the unit cell and the atomic positions are evolved according to the metadynamical equations of motion. We have found that the application of hydrostatic and c axis uniaxial pressure induces a phase transition from the magnetically ordered orthorhombic phase to the non-magnetic collapsed tetragonal phase in both BaFe2As2 and CaFe2As2. In the case of BaFe2As2, an intermediate tetragonal non-magnetic tetragonal phase is observed in addition. Application of the uniaxial pressure parallel to the c axis reduces the critical pressure of the phase transition by an order of magnitude, in agreement with the experimental findings. The in-plane pressure application did not result in transition to the non-magnetic tetragonal phase and instead, rotation of the magnetic order direction could be observed. This is discussed in the context of Ginzburg-Landau theory. We have also found that the magnetostructural phase transition is accompanied by a change in the Fermi surface topology, whereby the hole cylinders centered around the Gamma point disappear, restricting the possible Cooper pair scattering channels in the tetragonal phase. Our calculations also permit us to estimate the bulk moduli and the orthorhombic elastic constants of BaFe2As2 and CaFe2As2.
To study the electronic structure in systems with broken translational symmetry, such as doped iron based superconductors, it is necessary to develop a method to unfold the complicated bandstructures arising from the supercell calculations. In this thesis we present the unfolding method based on group theoretical techniques. We achieve the unfolding by employing induced irreducible representations of space groups. The unique feature of our method is that it treats the point group operations on an equal footing with the translations. This permits us to unfold the bandstructures beyond the limit of translation symmetry and also formulate the tight-binding models of reduced dimensionality if certain conditions are met. Inclusion of point group operations in the unfolding formalism allows us to reach important conclusions about the two versus one iron picture in iron based superconductors.
And finally, we present the results of ab-initio structure prediction in the cases of giant volume collapse in MnS2 and alkaline doped picene. In the case of MnS2, a previously unobserved high pressure arsenopyrite structure of MnS2 is predicted and stability regions for the two competing metastable phases under pressure are determined. In the case of alkaline doped picene, crystal structures with different levels of doping were predicted and used to study the role of electronic correlations.
This work derived the value of α-induced production cross sections of 77Kr and 77Br at α-energies of 12 MeV and 14 MeV, the thick target yields of 77Kr and 77Br at α-energies of 11.19 MeV, 13 MeV and 15.1 MeV and the thick target yield of 80Br as well as 80mBr at an α-energy of 15.1 MeV using the activation technique...
In dieser Arbeit wird der Strahltransport in einer Niederenergietransportsektion (LEBT) untersucht. Die Untersuchungen werden für die Betriebsmodi der im Aufbau befindlichen Neutronenquelle FRANZ an der Frankfurter Goethe-Universität durchgeführt. Hierbei wird die Akzeptanz eines Choppersystems nach der ersten Sektion des Transportwegs sowie die Akzeptanz des auf die zweite Sektion folgenden RFQ betrachtet und bestmöglich erfüllt. Die Auswirkungen durch die Raumladungswirkung des Ionenstrahls werden berücksichtigt, ebenso die mögliche thermische Belastung durch Strahlverlust an den Komponenten entlang des Strahlwegs. Weiterhin wird der Einfluss eines nicht optimierten Einschusses in den RFQ und die sich daraus ergebenden Strahleigenschaften am Ende des RFQs untersucht.
Eines der wichtigsten Experimente für Kernstrukturforschung und Messung stellarer Reaktionsraten ist das R3B-Experiment im Rahmen des FAIR-Projekts am GSI Helmholtzzentrum für Schwerionenforschung in Darmstadt. Der experimentelle Aufbau von R3B besteht aus mehreren einzelnen Teilchendetektoren für verschiedene Teilchensorten (Neutronen, Protonen, Spallationsund Spaltprodukte, Gammastrahlen), die alle möglichst vollständig detektiert und gemessen werden müssen. Für die Identifikation und Energiemessung schwerer, geladener Reaktionsprodukte ist eine sogenannte Time-of-Flight-Wall (Flugzeitwand) nötig. Der Name ergibt sich aus der Hauptaufgabe, der Flugzeitmessung für die Energiebestimmung der Teilchen, sowie der Geometrie eines solchen Detektors. Die in vorherigen Aufbauten verwendeten Detektoren diesen Typs erfüllen noch nicht die Anforderungen, die die Forschungsziele des R3B-Experiments stellen, daher wurde ein neues Design basierend auf Plastikszintillatoren entwickelt.
Für diese Arbeit wurde die theoretisch erreichbare Zeitauflösung des neuen Designs abgeschätzt sowie Testmessungen mit verschiedenen experimentellen Setups durchgeführt. Insbesondere wurde ein Prototyp der ToF-Wand im Rahmen einer Strahlzeit an der Beschleunigeranlage der GSI getestet. Die Ergebnisse dieser Messungen mit einem 58Ni28+-Strahl wurden im Hinblick auf Energie-, Zeit- und Ladungsauflösung sowie die Stabilität dieser Werte bei hohen Raten ausgewertet und so ein erster Eindruck von der Leistungsfähigkeit des Detektors und der Ausleseelektronik gewonnen und Einschränkungen und nötige Verbesserungen erkannt.
Zunächst sind einige Methoden und Techniken zusammenfassend aufzuzählen, welche mir in meiner Zeit am IKF nahegebracht wurden.
Von technischer Seite her sind hier der Umgang mit der Instituts-eigenen Lichtmikroskop und den pA-Messgeräten sowie der analogen Messkette zu nennen. Außerdem gegebenen GEM-Folien auf Fehlstellen zu untersuchen, sie unter Spannung zu testen und anschließen in die Testkammer zu montieren und diese anschließend ordnungsgemäß in Betrieb zu nehmen. Während des Betriebs der Kammer sind neben den Messungen selbst auch die Programmierung in C++ um ein vorhandenes GUI zu verstehen und erweitern zu können zu nennen. In der Analyse der gewonnenen Daten ist vor allem die im Institut verbreiteten Analyse-Software „Root“ zu nennen um Daten zu verarbeiten, zu plotten und zu fitten.
Der physikalische Gehalt der Messungen war in Folge der ersten Messung nicht mit Sicherheit zu bestimmen, da die Raten-Abhängigkeit des IB entweder grundlegender physikalischer oder technischer Natur sein konnte, was näher zu untersuchen blieb. Nach wiederholter Messung mit größerem Messbereich und einer zweiten Messreihe mit einer anderen Gas-Mischung konnten jedoch Aussagen getroffen werden.
So konnte in der Argon-Messung die gleiche Raten-Abhängigkeit des IBF wie zuvor festgestellt werden, während der IBF in der Neon-Mischung kaum merklich anstieg. Außerdem ist festzuhalten, dass Messungen an der Kathode nur über 10 pA problemlos genau sind. Darunter werden die Werte bei zu wenig Messzeit weniger aussagekräftig.
In dieser Arbeit wurde die automatisierte Separation von Heliummono-, -di- und -trimeren beschrieben. Unter Nutzung ihrer unterschiedlichen De-Broglie-Wellenlängen wurden die verschiedenen Fraktionen mit einem Nanogitter getrennt. Zunächst wurden einige physikalische Grundlagen zu den genannten Atom- bzw. Molekülspezies, der hier auftretenden Bindungsform der Van-der-Waals-Bindung und insbesondere zur Materiewellenbeugung gelegt. Anschließend wurde der Versuchsaufbau dargestellt.
Bei der Durchführung wurden zunächst die drei jeweils vorhandenen Gitter und Spalte zu je einer Messung kombiniert und die beste Kombination für die weiteren Messungen ausgewählt. Das Experiment wurde weitergeführt, indem für verschiedene Temperaturen und Quelldrücke jeweils ein Beugungsspektrum von der für alle Heliumteilchen identischen nullten Ordnung bis zur ersten Ordnung der Heliummonomere aufgenommen wurde.
In der Auswertung wurde die Detektionswahrscheinlichkeit auf rund 37 % abgeschätzt. Weiterhin wurden die Ereignisse in den ersten Maxima der einzelnen Heliumfraktionen gezählt und so unter Verwendung der Detektionswahrscheinlichkeit molare Konzentrationen für das Heliumdi- und -trimer berechnet. Dabei wurden Anteile von bis zu 0,45 % für das Heliumdimer und 4,2 % für das Heliumtrimer erreicht. Diese Molanteile und ihre Abhängigkeit von Druck und Temperatur stimmen qualitativ gut mit der Literatur überein, quantitativ lassen sie sich u. a. wegen abweichender Nachweismethoden kaum vergleichen.
Anschließend wurde der Abstand von Düse und Skimmer variiert mit dem Ergebnis, daß eine Veränderung im betrachteten Bereich keinen nennenswerten Einfluß auf die Bildungsraten von Di- und Trimeren hat. Weiterhin wurde die auf zweierlei Weise bstimmbare Geschwindigkeit der Heliumteilchen im Gasjet ermittelt und verglichen.
Die beiden Geschwindigkeiten weichen lediglich im unteren Temperaturbereich signifikant voneinander ab, wofür plausible Erklärungsansätze dargelegt wurden.
Die Größe der Quellregion der betrachteten Heliumcluster wurde unter geometrischen Gesichtspunkten und unter Extrapolation der für verschiedene Spaltbreiten gemessenen Maximumsbreiten untersucht. Im Ergebnis wird die Quellbreite zu 58,5 μm abgeschätzt.
Die Automatisierung des Aufbaus erlaubte eine Vielzahl von systematischen Messungen, die ohne diese Automatisierung sehr zeitaufwendig gewesen wären. Insbesondere wurden in kurzer Zeit - wie zuvor geschildert - die Beugungsmuster von drei Gittern in Kombination mit je drei verschiedenen Kollimationspalten sowie die Abhängigkeit der Heliumdimer- und -trimerbildung von Temperatur, Druck und Abstand von Düse und Skimmer untersucht. Die Automatisierung erlaubt für zukünftige Messungen, z. B. in Strahlzeiten am Freien Elektronenlaser FLASH, jeweils in situ die Clusterbildung zu untersuchen. Möge das beschriebene Experiment nicht nur diese, sondern auch viele weitere Messungen beschleunigen helfen und so zum gesellschaftlichen Erkenntnisgewinn beitragen!