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Towards the goal to understand the role of land-surface processes over the Indian sub-continent, a series of soil-moisture sensitivity simulations have been performed using a non-hydrostatic regional climate model COSMO-CLM. The experiments were driven by the lateral boundary conditions provided by the ERA-Interim (ECMWF) reanalysis. The simulation results show that the pre-monsoonal soil moisture has a significant influence on the monsoonal precipitation. Both, positive and negative soil-moisture precipitation (S-P) feedback processes are of importance. The negative S-P feedback process is especially influential in the western and the northern parts of India.
Seit nunmehr 20 Jahren findet regelmäßig alle zwei Jahre das Symposium "Tektonik — Strukturgeologie — Kristallingeologie" (TSK) statt. Die Tagung soll insbesondere jungen Nachwuchswissenschaftlern die Möglichkeit bieten, ihre Ergebnisse zu diskutieren und einem breiten Fachpublikum vorzustellen. Dies ist natürlich besonders attraktiv, wenn auch die ‚alten Hasen‘ der Zunft eifrig dabei sind.
In diesem Jahr wird schon TSK 11 — nach Tübingen, Erlangen, Graz, Frankfurt, Salzburg, Freiberg, Freiburg und Aachen nun zum zweiten Mal nach 1994 wieder in Göttingen durchgeführt. Wir freuen uns, auch dieses Mal wieder ein vielseitiges Tagungsprogramm präsentieren zu können. Die vorgestellten Arbeiten befassen sich mit Geländebeobachtungen, Laboranalysen und -experimenten bis hin zu Computermodellierungen. Im Maßstab reichen sie vom submikroskopischen Bereich bis hin zu ganzen Orogenen. Dabei werden sowohl duktile als auch spröde Deformationsprozesse beleuchtet. Regionale Geologie ist ebenso Thema wie auch eher angewandte Fragestellungen.
Um die einzelnen Beiträge schnell auffinden zu können, wurden diese alphabetisch nach Erstautoren geordnet. Aus Zeitgründen konnte nur der kleinere Teil der mehr als einhundert eingegangen Beiträge in das Vortragsprogramm aufgenommen werden. Auf parallele Vortragssitzungen haben wir bewusst verzichtet. Besonderen Raum für anregende Diskussionen sollen auch die thematisch zusammengestellten Postersitzungen bieten, für die wir spezielle Zeiten eingeräumt haben. Hierzu werden Poster jeweils vorher im Plenum kurz vorgestellt.
Die eingegangenen Manuskripte wurden, wie bei TSK üblich, für die Publikation keinem Gutachterverfahren unterzogen. Daher sind die jeweiligen Autoren allein für den Inhalt verantwortlich. ...
Geoprax : Newsletter
(1999)
Nölscher, Anke Christine ; Bourtsoukidis, Efstratios ; Bonn, Boris ; Kesselmeier, Jürgen ; Lelieveld, Johannes ; Williams, Jonathan
Numerous reactive volatile organic compounds (VOCs) are emitted into the atmosphere by vegetation. Most biogenic VOCs are highly reactive towards the atmosphere's most important oxidant, the hydroxyl (OH) radical. One way to investigate the chemical interplay between biosphere and atmosphere is through the measurement of total OH reactivity, the total loss rate of OH radicals. This study presents the first determination of total OH reactivity emission rates (measurements via the Comparative Reactivity Method) based on a branch cuvette enclosure system mounted on a Norway spruce (Picea abies) throughout spring, summer and autumn 2011. In parallel separate VOC emission rates were monitored by a Proton Transfer Reaction-Mass Spectrometer (PTR-MS), and total ozone (O3) loss rates were obtained inside the cuvette. Total OH reactivity emission rates were in general temperature and light dependent, showing strong diel cycles with highest values during daytime. Monoterpene emissions contributed most, accounting for 56–69% of the measured total OH reactivity flux in spring and early summer. However, during late summer and autumn the monoterpene contribution decreased to 11–16%. At this time, a large missing fraction of the total OH reactivity emission rate (70–84%) was found when compared to the VOC budget measured by PTR-MS. Total OH reactivity and missing total OH reactivity emission rates reached maximum values in late summer corresponding to the period of highest temperature. Total O3 loss rates within the closed cuvette showed similar diel profiles and comparable seasonality to the total OH reactivity fluxes.
Total OH reactivity fluxes were also compared to emissions from needle storage pools predicted by a temperature-only dependent algorithm. Deviations of total OH reactivity fluxes from the temperature-only dependent emission algorithm were observed for occasions of mechanical and heat stress. While for mechanical stress, induced by strong wind, measured VOCs could explain total OH reactivity emissions, during heat stress they could not. The temperature driven algorithm matched the diel course much better in spring than in summer, indicating a different production and emission scheme for summer and early autumn. During these times, unmeasured and possibly unknown primary biogenic emissions contributed significantly to the observed total OH reactivity flux.
A complete, well-preserved record of the Cenomanian/Turonian (C/T) Oceanic Anoxic Event 2 (OAE-2) was recovered from Demerara Rise in the southern North Atlantic Ocean (ODP site 1260). Across this interval, we determined changes in the stable carbon isotopic composition of sulfur-bound phytane (δ13Cphytane), a biomarker for photosynthetic algae. The δ13Cphytane record shows a positive excursion at the onset of the OAE-2 interval, with an unusually large amplitude (~7‰) compared to existing C/T proto-North Atlantic δ13Cphytane records (3–6‰). Overall, the amplitude of the excursion of δ13Cphytane decreases with latitude. Using reconstructed sea surface temperature (SST) gradients for the proto-North Atlantic, we investigated environmental factors influencing the latitudinal δ13Cphytane gradient. The observed gradient is best explained by high productivity at DSDP Site 367 and Tarfaya basin before OAE-2, which changed in overall high productivity throughout the proto-North Atlantic during OAE-2. During OAE-2, productivity at site 1260 and 603B was thus more comparable to the mid-latitude sites. Using these constraints as well as the SST and δ13Cphytane-records from Site 1260, we subsequently reconstructed pCO2 levels across the OAE-2 interval. Accordingly, pCO2 decreased from ca. 1750 to 900 ppm during OAE-2, consistent with enhanced organic matter burial resulting in lowering pCO2. Whereas the onset of OAE-2 coincided with increased pCO2, in line with a volcanic trigger for this event, the observed cooling within OAE-2 probably resulted from CO2 sequestration in black shales outcompeting CO2 input into the atmosphere. Together these results show that the ice-free Cretaceous world was sensitive to changes in pCO2 related to perturbations of the global carbon cycle.
Mit dem mathematischen Werkzeug zur Filterung von Lärmprozessen, die für die Praktizierung der numerischen Wettervorhersage in ihrer Anfangszeit eine große Rolle gespielt hat, wird an den linearisierten Gleichungen für ein barotropes Flachwassermodell im β-Format die Frage behandelt, wie sich der Rossby-förmige Wellenmodus entwickelt, wenn gleichzeitige Trägheitsschwerewellenmoden infolge von veränderlichen filternden Gleichungen unterdrückt werden.
Zunächst werden einige analytische Grundbeziehungen einer lärmfreien Adjustierung von Anfangsfeldern ausgeführt. Dann richtet sich die Untersuchung auf lärmfilternde prognostische Modellgleichungen (Absch. 5, 6, 7). Aus dieser Analysis in Abhängigkeit von der Filterstufe findet man im Vergleich mit der konventionellen synoptisch-skaligen Rossby-Formel, die der Filterstufe Null entspricht, zum Teil erweiterte Wellengeschwindigkeiten der Rossby-förmigen Physik. Dabei treten sogar unerwartete neue Effekte auf, die wohl primär im Langwellenspektrum zählen.
wo assumptions underlie current models of the geographical ranges of perennial plant species: 1. current ranges are in equilibrium with the prevailing climate, and 2. changes are attributable to changes in macroclimatic factors, including tolerance of winter cold, the duration of the growing season, and water stress during the growing season, rather than to biotic interactions. These assumptions allow model parameters to be estimated from current species ranges. Deterioration of growing conditions due to climate change, e.g. more severe drought, will cause local extinction. However, for many plant species, the predicted climate change of higher minimum temperatures and longer growing seasons means, improved growing conditions. Biogeographical models may under some circumstances predict that a species will become locally extinct, despite improved growing conditions, because they are based on an assumption of equilibrium and this forces the species range to match the species-specific macroclimatic thresholds. We argue that such model predictions should be rejected unless there is evidence either that competition influences the position of the range margins or that a certain physiological mechanism associated with the apparent improvement in growing conditions negatively affects the species performance. We illustrate how a process-based vegetation model can be used to ascertain whether such a physiological cause exists. To avoid potential modelling errors of this type, we propose a method that constrains the scenario predictions of the envelope models by changing the geographical distribution of the dominant plant functional type. Consistent modelling results are very important for evaluating how changes in species areas affect local functional trait diversity and hence ecosystem functioning and resilience, and for inferring the implications for conservation management in the face of climate change.
Recently, new soil data maps were developed, which include vertical soil properties like soil type. Implementing those into a multilayer Soil-Vegetation-Atmosphere-Transfer (SVAT) scheme, discontinuities in the water content occur at the interface between dissimilar soils. Therefore, care must be taken in solving the Richards equation for calculating vertical soil water fluxes. We solve a modified form of the mixed (soil water and soil matric potential based) Richards equation by subtracting the equilibrium state of soil matrix potential ψE from the hydraulic potential ψh. The sensitivity of the modified equation is tested under idealized conditions. The paper will show that the modified equation can handle with discontinuities in soil water content at the interface of layered soils.
Duplissy, Jonathan ; DeCarlo, Peter F. ; Dommen, Josef ; Alfarra, M. Rami ; Metzger, Axel ; Barmpadimos, Iakovos ; Prevot, André Stephan Henry ; Weingartner, Ernest ; Tritscher, Torsten ; Gysel, Martin ; Aiken, Allison C. ; Jimenez, Jose Luis ; Canagaratna, Manjula R. ; Worsnop, Douglas R. ; Collins, Donald R. ; Tomlinson, Jason M. ; Baltensperger, Urs
A hygroscopicity tandem differential mobility analyzer (HTDMA) was used to measure the water uptake (hygroscopicity) of secondary organic aerosol (SOA) formed during the chemical and photochemical oxidation of several organic precursors in a smog chamber. Electron ionization mass spectra of the non-refractory submicron aerosol were simultaneously determined with an aerosol mass spectrometer (AMS), and correlations between the two different signals were investigated. SOA hygroscopicity was found to strongly correlate with the relative abundance of the ion signal m/z 44 expressed as a fraction of total organic signal (f44). m/z 44 is due mostly to the ion fragment CO2+ for all types of SOA systems studied, and has been previously shown to strongly correlate with organic O/C for ambient and chamber OA. The analysis was also performed on ambient OA from two field experiments at the remote site Jungfraujoch, and the megacity Mexico City, where similar results were found. A simple empirical linear relation between the hygroscopicity of OA at subsaturated RH, as given by the hygroscopic growth factor (GF) or "ϰorg" parameter, and f44 was determined and is given by ϰorg = 2.2 × f44 − 0.13. This approximation can be further verified and refined as the database for AMS and HTDMA measurements is constantly being expanded around the world. The use of this approximation could introduce an important simplification in the parameterization of hygroscopicity of OA in atmospheric models, since f44 is correlated with the photochemical age of an air mass.
Duplissy, Jonathan ; DeCarlo, Peter F. ; Dommen, Josef ; Alfarra, M. Rami ; Metzger, Axel ; Barmpadimos, Iakovos ; Prevot, André Stephan Henry ; Weingartner, Ernest ; Tritscher, Torsten ; Gysel, Martin ; Aiken, Allison C. ; Jimenez, Jose Luis ; Canagaratna, Manjula R. ; Worsnop, Douglas R. ; Collins, Donald R. ; Tomlinson, Jason M. ; Baltensperger, Urs
A hygroscopicity tandem differential mobility analyzer (HTDMA) was used to measure the water uptake (hygroscopicity) of secondary organic aerosol (SOA) formed during the chemical and photochemical oxidation of several organic precursors in a smog chamber. Electron ionization mass spectra of the non-refractory submicron aerosol were simultaneously determined with an aerosol mass spectrometer (AMS), and correlations between the two different signals were investigated. SOA hygroscopicity was found to strongly correlate with the relative abundance of the ion signal m/z 44 expressed as a fraction of total organic signal (f44). m/z 44 is due mostly to the ion fragment CO2+ for all types of SOA systems studied, and has been previously shown to strongly correlate with organic O/C for ambient and chamber OA. The analysis was also performed on ambient OA from two field experiments at the remote site Jungfraujoch, and the megacity Mexico City, where similar results were found. A simple empirical linear relation between the hygroscopicity of OA at subsaturated RH, as given by the hygroscopic growth factor (GF) or "κorg" parameter, and f44 was determined and is given by κorg=2.2×f44−0.13. This approximation can be further verified and refined as the database for AMS and HTDMA measurements is constantly being expanded around the world. The use of this approximation could introduce an important simplification in the parameterization of hygroscopicity of OA in atmospheric models, since f44 is correlated with the photochemical age of an air mass.
Niedermeier, Dennis ; Hartmann, Susan ; Clauss, Tina ; Wex, Heike ; Kiselev, Alexei ; Sullivan, Ryan C. ; DeMott, Paul J. ; Petters, Markus D. ; Reitz, Paul ; Schneider, Johannes ; Mikhailov, Eugene ; Sierau, Berko ; Stetzer, Olaf ; Reimann, Bernd ; Bundke, Ulrich ; Shaw, Raymond A. ; Buchholz, Angela ; Mentel, Thomas F. ; Stratmann, Frank
Niedermeier, Dennis ; Hartmann, Susan ; Clauss, Tina ; Wex, Heike ; Kiselev, Alexei ; Sullivan, Ryan C. ; DeMott, Paul J. ; Petters, Markus D. ; Reitz, Paul ; Schneider, Johannes ; Mikhailov, Eugene ; Sierau, Berko ; Stetzer, Olaf ; Reimann, Bernd ; Bundke, Ulrich ; Shaw, Raymond A. ; Buchholz, Angela ; Mentel, Thomas F. ; Stratmann, Frank
During the measurement campaign FROST 2 (FReezing Of duST 2), the Leipzig Aerosol Cloud Interaction Simulator (LACIS) was used to investigate the influence of various surface modifications on the ice nucleating ability of Arizona Test Dust (ATD) particles in the immersion freezing mode. The dust particles were exposed to sulfuric acid vapor, to water vapor with and without the addition of ammonia gas, and heat using a thermodenuder operating at 250 °C. Size selected, quasi monodisperse particles with a mobility diameter of 300 nm were fed into LACIS and droplets grew on these particles such that each droplet contained a single particle. Temperature dependent frozen fractions of these droplets were determined in a temperature range between −40 °C ≤T≤−28 °C. The pure ATD particles nucleated ice over a broad temperature range with their freezing behavior being separated into two freezing branches characterized through different slopes in the frozen fraction vs. temperature curves. Coating the ATD particles with sulfuric acid resulted in the particles' IN potential significantly decreasing in the first freezing branch (T>−35 °C) and a slight increase in the second branch (T≤−35 °C). The addition of water vapor after the sulfuric acid coating caused the disappearance of the first freezing branch and a strong reduction of the IN ability in the second freezing branch. The presence of ammonia gas during water vapor exposure had a negligible effect on the particles' IN ability compared to the effect of water vapor. Heating in the thermodenuder led to a decreased IN ability of the sulfuric acid coated particles for both branches but the additional heat did not or only slightly change the IN ability of the pure ATD and the water vapor exposed sulfuric acid coated particles. In other words, the combination of both sulfuric acid and water vapor being present is a main cause for the ice active surface features of the ATD particles being destroyed. A possible explanation could be the chemical transformation of ice active metal silicates to metal sulfates. The strongly enhanced reaction between sulfuric acid and dust in the presence of water vapor and the resulting significant reductions in IN potential are of importance for atmospheric ice cloud formation. Our findings suggest that the IN concentration can decrease by up to one order of magnitude for the conditions investigated.
Niedermeier, Dennis ; Hartmann, Susan ; Clauss, Tina ; Wex, Heike ; Kiselev, Alexei ; Sullivan, Ryan C. ; DeMott, Paul J. ; Petters, Markus D. ; Reitz, Paul ; Schneider, Johannes ; Mikhailov, Eugene ; Sierau, Berko ; Stetzer, Olaf ; Reimann, Bernd ; Bundke, Ulrich ; Shaw, Raymond A. ; Buchholz, Angela ; Mentel, Thomas F. ; Stratmann, Frank
During the measurement campaign FROST 2 (FReezing Of duST 2), the Leipzig Aerosol Cloud Interaction Simulator (LACIS) was used to investigate the influences of various surface modifications on the immersion freezing behavior of Arizona Test Dust (ATD) particles. The dust particles were exposed to sulfuric acid vapor, to water vapor with and without the addition of ammonia gas, and heat using a thermodenuder operating at 250 °C. Size selected, quasi monodisperse particles with a mobility diameter of 300 nm were fed into LACIS and droplets grew on these particles such that each droplet contained a single particle. Temperature dependent frozen fractions of these droplets were determined in a temperature range between −40 °C ≤ T ≤ −28 °C. The pure ATD particles nucleated ice over a~broad temperature range with their freezing behavior being separated into two freezing branches characterized through different slopes in the frozen fraction vs. temperature curves. Coating the ATD particles with sulfuric acid resulted in the particles' IN potential significantly decreasing in the first freezing branch (T > −35 °C) and a slight increase in the second branch (T≤ −35 °C). The addition of water vapor after the sulfuric acid coating caused the disappearance of the first freezing branch and a strong reduction of the IN ability in the second freezing branch. The presence of ammonia gas during water vapor exposure had a negligible effect on the particles' IN ability compared to the effect of water vapor. Heating in the thermodenuder led to a decreased IN ability of the sulfuric acid coated particles for both branches but the additional heat did not or only slightly change the IN ability of the pure ATD and the water vapor exposed sulfuric acid coated particles. In other words, the combination of both sulfuric acid and water vapor being present is a main cause for the ice active surface features of the ATD particles being destroyed. A possible explanation could be the chemical transformation of ice active metal silicates to metal sulfates. From an atmospheric point of view, and here specifically the influences of atmospheric aging on the IN ability of dust particles, the strongly enhanced reaction between sulfuric acid and dust in the presence of water vapor, and the resulting significant reductions in IN potential, are certainly very interesting.
Bingemer, Heinz ; Klein, Holger ; Ebert, Martin ; Haunold, Werner ; Bundke, Ulrich ; Herrmann, Thomas ; Kandler, Konrad ; Müller-Ebert, Dörthe ; Weinbruch, Stephan ; Judt, Anna ; Weber, A. ; Nillius, Björn ; Ardon-Dryer, Karin ; Levin, Zev ; Curtius, Joachim
We have sampled atmospheric ice nuclei (IN) and aerosol in Germany and in Israel during spring 2010. IN were analyzed by the static vapor diffusion chamber FRIDGE, as well as by electron microscopy. During the Eyjafjallajökull volcanic eruption of April 2010 we have measured the highest ice nucleus number concentrations (>600 l−1) in our record of 2 yr of daily IN measurements in central Germany. Even in Israel, located about 5000 km away from Iceland, IN were as high as otherwise only during desert dust storms. The fraction of aerosol activated as ice nuclei at −18 °C and 119% rhice and the corresponding area density of ice-active sites per aerosol surface were considerably higher than what we observed during an intense outbreak of Saharan dust over Europe in May 2008.
Pure volcanic ash accounts for at least 53–68% of the 239 individual ice nucleating particles that we collected in aerosol samples from the event and analyzed by electron microscopy. Volcanic ash samples that had been collected close to the eruption site were aerosolized in the laboratory and measured by FRIDGE. Our analysis confirms the relatively poor ice nucleating efficiency (at −18 °C and 119% ice-saturation) of such "fresh" volcanic ash, as it had recently been found by other workers. We find that both the fraction of the aerosol that is active as ice nuclei as well as the density of ice-active sites on the aerosol surface are three orders of magnitude larger in the samples collected from ambient air during the volcanic peaks than in the aerosolized samples from the ash collected close to the eruption site. From this we conclude that the ice-nucleating properties of volcanic ash may be altered substantially by aging and processing during long-range transport in the atmosphere, and that global volcanism deserves further attention as a potential source of atmospheric ice nuclei.