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This paper reports calculations of the influence of a reaction time T>10-21 s in deep-inelastic Xe-Pb collisions on the energy spectrum of δ electrons ejected in the same collision. It is shown that the lifetime of the superheavy composite system causes pronounced oscillations of width ε=h/T in the electron distribution, which survive the inclusion of multistep excitations and the folding with a lifetime distribution function. This effect may serve as an atomic clock for deep-inelastic collisions.
This Letter discusses inner-shell excitation in collisions of very heavy ions (Z1+Z2≳140) in the framework of the quasimolecular model. The importance of multistep excitations and of coupling between continuum states is demonstrated. The 1sσ vacancy probabilities resulting from coupled-channels calculations exceed perturbation theory by a factor 3-5, thus giving good agreement with recent experimental results.
Binding energies and wave functions of inner-shell electronic states in superheavy quasimolecules with (Zp+Zt)α>1 are calculated. Ionization during a collision of very heavy ions is investigated within a molecular basis generated by the solutions of the two-center Dirac equation. Transitions to vacant bound states as well as direct excitation to the continuum are taken into account. We present theoretical values for the ionization probability as a function of impact parameter, bombarding energy, and combined nuclear charge. Our computed results are compared with recent experimental data. It is suggested that relativistic binding energies of electrons in superheavy quasimolecules can be determined experimentally via the impact-parameter dependence of ionization and the anisotropy of quasimolecular radiation.
Within an extended semiquantal theory we perform large-sized coupled-channel calculations involving 260 collective levels for Coulomb fission of 238U. Differential Coulomb fission cross sections are studied as a function of bombarding energy and impact parameter for several projectiles. In the Xe + U case, total cross sections are also given. We find a strong dependence on projectile charge number, PCF(180°)∼(Zp)6 in the region 50≤Zp≤92 for a fixed ratio E/ECoul, which might be helpful to separate Coulomb fission experimentally from sequential fission following transfer reactions. Since the cross sections are sensitive to the moment of inertia ⊖ at the saddle point, Coulomb fission can serve as a tool to investigate the dependence of ⊖ on elongation. The fragment angular distribution exhibits deviations from 1/sinθf which are pronounced at low incident energies. Our theory indicates that the recently measured Xe + U fission cross sections contain a major fraction of Coulomb-induced fission at E≤0.85 ECoul. NUCLEAR REACTIONS, FISSION Calculated Coulomb fission cross sections σ(Ep,θp) for 54Xe, 67Ho, 82Pb, 92U→92238U, fragment angular distribution, fission energy spectrum, mean spin value 〈Jf〉.
The theory of nucleon transfer in heavy ion reactions is formulated on the basis of the molecular particlecore model for a system consisting of two cores and one extracore nucleon. The extracore nucleon is described by the molecular wave functions of the asymmetric two-center shell model. The cores, which are assumed to be collectively excitable, are treated with vibrator-rotator models. Potentials for shape polarization are contained in the asymmetric two-center shell model and the interaction between the cores. The excitation and transfer of the extracore nucleon is induced by the radial and rotational couplings. The coupled channel equations, which include the recoil effects in first approximation, are derived in a form suitable for numerical calculations of cross sections. NUCLEAR REACTIONS Heavy ion scattering, theory of nucleon transfer, molecular wave functions, two-center shell model, collective and single-particle excitation.
Inner-shell ionization induced by nuclear Coulomb excitation in collisions of very heavy ions
(1978)
K- and L-shell ionization of 238U with Xe and U projectiles is investigated. Internal conversion following nuclear Coulomb excitation which is particularly important for deformed heavy nuclei is compared with direct ionization of inner-shell electrons in superheavy quasimolecules. Both processes exhibit different impact-parameter dependences. As a result of internal conversion, about 0.1-0.3 K holes per central collision are created.
On the basis of the two-center shell model a theory is developed for the excitation of loosely bound nucleons in heavy ion collisions. These nucleons move in the two-center shell model potential generated by all the nucleons and are described by molecular wave functions. The model is applied to calculate the cross sections for the elastic and inelastic 13C-13C scattering. The cross sections show intermediate structures caused by the excitation of quasibound resonances in the molecular nucleus-nucleus potential. NUCLEAR REACTIONS 13C(13C,13C) molecular wave functions, dynamical two-center shell model, quasimolecular resonances, radial and Coriolis coupling, coupled channel calculations for σ(θ).
Quasimolecular resonance structures in the 12C-12C system are studied in the framework of the coupled channel formalism in the energy range Ec.m.=5-14 MeV. The influence of the coupling of the first excited 2+ state in 12C on the resonance structures is investigated by choosing various types of coupling potentials. The intermediate structures in the reflection and transition coefficients and cross sections can be interpreted with the double resonance mechanism. NUCLEAR REACTIONS 12C(12C, 12C), quasimolecular states, coupling potentials, coupled channel calculations for σ(θ).
The theory of direct electron-positron pair production in the collision of heavy ions is formulated in the framework of the quasimolecular model. The pair production process acquires a collective nature for (Z1+Z2)α>1 and can be understood as the shakeoff of the strong vacuum polarization cloud formed in the quasimolecule. The total cross section is, e.g., 76 μb for Pb + Pb at Coulomb barrier energies.
Internal conversion of γ rays from Coulomb-excited nuclear levels cannot be neglected compared with the spontaneous and induced positron production in overcritical electric fields. It is shown that both processes are separable by their different distributions with respect to the ion angle and the positron energy.
We show that information about quasimolecular electronic binding energies in transient atomic systems of Z=Z1+Z2 up to 184 can be obtained from three sources: (1) the impact-parameter dependence of the ionization probability; (2) the ionization probability in head-on collisions as a function of total nuclear charge Z; (3) the delta-electron spectrum in coincidence with K-vacancy formation in asymmetric collisions. Experiments are proposed and discussed.
Determination of the effective 12C + 12C potential from the sub-Coulomb single-particle resonances
(1974)
The sub-Coulomb resonances observed in the total reaction yield of the 12C + 12C system at 4.9, 5.6, and 6.2 MeV are explained as single-particle resonances. The "true" effective 12C + 12C potential is determined directly as the real potential which reproduces best the position and the spacing of the observed sub-Coulomb resonances. This potential is found from a parametrization of the two limiting adiabatic and sudden potentials.
the development of the mass asymmetry vibrations in the final stages of the fission process is studied with an approximate treatment of the coupling to relative motion. A parametrized friction is introduced and its effects are studied. Numerical results are presented for 236U, together with estimates for the kinetic energy of the fragments. RADIOACTIVITY, FISSION 236U; calculated mass distribution, kinetic energy distribution. Collective dynamics, shell correction method, cranking model.
It is shown that nuclear matter is compressed during the encounter of heavy ions. If the relative velocity of the nuclei is larger than the velocity of first sound in nuclear matter (compression sound for isospin T=0), nuclear shock waves occur. They lead to densities which are 3-5 times higher than the nuclear equilibrium density ρ0, depending on the energy of the nuclei. The implications of this phenomenon are discussed.
The mechanisms of spontaneous and induced emission of radiation are derived from the Dirac equation in a rotating coordinate system. The molecular-orbital x-ray spectra exhibit a strong asymmetry with respect to the beam axis. The asymmetry peaks for the high-energy transitions, which can be used for spectroscopy of two-center orbitals.
In critical or nearly critical heavy-ion collisions, induced as well as spontaneous energyless e-e+ pair creation result in the decay of the neutral vacuum. Induced transitions from the negative-energy continuum into a vacant molecular 1s level can occur even in the absence of diving and produce a substantial enhancement and broadening of the previously considered spontaneous positron spectrum. Total cross sections of 5 b have been calculated for U-U collisions.
With the mass asymmetry described by the dynamical collective fragmentation coordinate ξ, and with use of the asymmetric two-center shell model, the fission mass distributions for 226Ra, 236U, and 258Fm (which are typical representatives for triple-, double-, and single-humped distributions) are explained.
In view of new high-precision experiments in atomic physics it seems necessary to reexamine nonlinear theories of electrodynamics. The precise calculation of electronic and muonic atomic energies has been used to determine the possible size of the upper limit Emax to the electric field strength, which has been assumed to be a parameter. This is opposed to Born's idea of a purely electromagnetic origin of the electron's mass which determines Emax. We find Emax≥1.7×1020 V/cm.