Trapping, chemistry and export of trace gases in the South Asian summer monsoon observed during CARIBIC flights in 2008

  • The CARIBIC (Civil Aircraft for the Regular Investigation of the Atmosphere Based on an Instrument Container) passenger aircraft observatory performed in situ measurements at 10–12 km altitude in the South Asian summer monsoon anticyclone between June and September 2008. These measurements enable us to investigate this atmospheric region, which so far has mostly been observed from satellites, using the broad suite of trace gases and aerosols measured by CARIBIC. Elevated levels of a range of atmospheric pollutants were recorded e.g. carbon monoxide, total reactive nitrogen oxides, aerosol particles and several volatile organic compounds. The measurements provide detailed information about the chemical composition of air in different parts of the monsoon anticyclone, particularly of ozone precursors. While covering a range of 3500 km inside the monsoon anticyclone, CARIBIC observations show remarkable consistency, i.e. with regular latitudinal patterns of trace gases during the entire monsoon period. Trajectory calculations indicate that these air masses originated mainly from South Asia and Mainland Southeast Asia. Using the CARIBIC trace gas and aerosol measurements in combination with the Lagrangian particle dispersion model FLEXPART we investigated the characteristics of monsoon outflow and the chemical evolution of air masses during transport. Estimated photochemical ages of the air were found to agree well with transport times from a source region east of 95 ° E. The photochemical ages of the air in the southern part of the monsoon anticyclone were consistently younger (less than 7 days) and the air masses mostly in an ozone forming chemical regime. In its northern part the air masses were older (up to 13 days) and had unclear ozone formation or destruction potential. Based on analysis of forward trajectories several receptor regions were identified. In addition to predominantly westward transport, we found evidence for efficient transport (within 10 days) to the Pacific and North America, particularly during June and September, and also of cross-tropopause exchange, which was strongest during June and July. Westward transport to Africa and further to the Mediterranean was the main pathway during July.

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Author:Armin Rauthe-Schöch, Angela Baker, Tanja J. SchuckORCiDGND, Carl Brenninkmeijer, Andreas Zahn, Markus Hermann, Greta StratmannGND, Helmut Ziereis, Peter F. J. van Velthoven, Jos Lelieveld
URN:urn:nbn:de:hebis:30:3-418866
URL:http://www.atmos-chem-phys-discuss.net/15/6967/2015
DOI:https://doi.org/10.5194/acpd-15-6967-2015
ISSN:1680-7367
ISSN:1680-7375
Parent Title (English):Atmospheric chemistry and physics. Discussions
Publisher:European Geosciences Union
Place of publication:Katlenburg-Lindau
Document Type:Article
Language:English
Date of Publication (online):2016/11/17
Date of first Publication:2015/03/10
Publishing Institution:Universitätsbibliothek Johann Christian Senckenberg
Release Date:2016/11/17
Volume:15
Page Number:52
First Page:6967
Last Page:7018
Note:
© Author(s) 2015. CC Attribution 3.0 License.
HeBIS-PPN:424009870
Institutes:Geowissenschaften / Geographie / Geowissenschaften
Dewey Decimal Classification:5 Naturwissenschaften und Mathematik / 55 Geowissenschaften, Geologie / 550 Geowissenschaften
Sammlungen:Universitätspublikationen
Licence (German):License LogoCreative Commons - Namensnennung 3.0