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RuO₂: a puzzle to be solved
(2023)
Altermagnetism is a topic that has lately been gaining attention and the RuO2 compound is among one of the most studied altermagnetic candidates. However, the survey of available literature on RuO2 properties suggests that there is no consensus about the magnetism of this material. By performing density functional theory calculations, we show that the electronic properties of stoichiometric RuO2 are described in terms of a smaller Hubbard U within DFT+U than the value required to have magnetism. We further argue that Ru vacancies can actually aid the formation of a magnetic state in RuO2. This in turn suggests that a characterization of the amount of Ru vacancies in experimental samples might help the resolution of the controversy between the different experimental results.
Binding energies and wave functions of inner-shell electronic states in superheavy quasimolecules with (Zp+Zt)α>1 are calculated. Ionization during a collision of very heavy ions is investigated within a molecular basis generated by the solutions of the two-center Dirac equation. Transitions to vacant bound states as well as direct excitation to the continuum are taken into account. We present theoretical values for the ionization probability as a function of impact parameter, bombarding energy, and combined nuclear charge. Our computed results are compared with recent experimental data. It is suggested that relativistic binding energies of electrons in superheavy quasimolecules can be determined experimentally via the impact-parameter dependence of ionization and the anisotropy of quasimolecular radiation.
We show that information about quasimolecular electronic binding energies in transient atomic systems of Z=Z1+Z2 up to 184 can be obtained from three sources: (1) the impact-parameter dependence of the ionization probability; (2) the ionization probability in head-on collisions as a function of total nuclear charge Z; (3) the delta-electron spectrum in coincidence with K-vacancy formation in asymmetric collisions. Experiments are proposed and discussed.
A careful investigation of different corrections to binding energies of electrons in almost critical fields is performed. We investigate quantitatively the influence of the nuclear charge parameters, nuclear mass, degree of ionization on the value of the critical charge of the nucleus. Rather qualitative arguments are given to establish the contribution of the quantumelectrodynamic corrections, which are found to be small. Some phenomenological modifications of QED are quantitatively investigated and found to be of negligible influence on the value of the critical field. For heavy ion collisions with Z1+Z2>Zcr the critical separations between ions are given as results of precise solutions of the relativistic two coulomb center problem. Corrections due to electron-electron interaction are considered. We find (with present theoretical accuracy) Zcr=173±2, in the heavy ion collisions Rcr(U-U) = 34.7±2 fm and Rcr (U-Cf)=47.7±2 fm. We shortly consider the possibility of spontaneous muon production in muonic supercritical fields.
Inner-shell ionization induced by nuclear Coulomb excitation in collisions of very heavy ions
(1978)
K- and L-shell ionization of 238U with Xe and U projectiles is investigated. Internal conversion following nuclear Coulomb excitation which is particularly important for deformed heavy nuclei is compared with direct ionization of inner-shell electrons in superheavy quasimolecules. Both processes exhibit different impact-parameter dependences. As a result of internal conversion, about 0.1-0.3 K holes per central collision are created.
In view of new high-precision experiments in atomic physics it seems necessary to reexamine nonlinear theories of electrodynamics. The precise calculation of electronic and muonic atomic energies has been used to determine the possible size of the upper limit Emax to the electric field strength, which has been assumed to be a parameter. This is opposed to Born's idea of a purely electromagnetic origin of the electron's mass which determines Emax. We find Emax≥1.7×1020 V/cm.
We calculate the spin polarization of 1sσ vacancies and emitted δ electrons induced by the strong magnetic field (|Bmax|∼1016G) in collisions of very heavy ions (Z1+Z2=178). The electron excitations are determined by the solution of coupled-channel equations within the quasimolecular basis states including the vector potential. The formulation is extended to the many-electron case. Spin polarizations of the order of 5-10% for impact energies below the Coulomb barrier are predicted.
The theory of direct electron-positron pair production in the collision of heavy ions is formulated in the framework of the quasimolecular model. The pair production process acquires a collective nature for (Z1+Z2)α>1 and can be understood as the shakeoff of the strong vacuum polarization cloud formed in the quasimolecule. The total cross section is, e.g., 76 μb for Pb + Pb at Coulomb barrier energies.
This paper reports calculations of the influence of a reaction time T>10-21 s in deep-inelastic Xe-Pb collisions on the energy spectrum of δ electrons ejected in the same collision. It is shown that the lifetime of the superheavy composite system causes pronounced oscillations of width ε=h/T in the electron distribution, which survive the inclusion of multistep excitations and the folding with a lifetime distribution function. This effect may serve as an atomic clock for deep-inelastic collisions.
The energy shift of K electrons in heavy atoms due to the self-energy correction has been calculated. This process is treated to all orders in Zα, where Z denotes the nuclear charge. For the superheavy system Z=170, where the K-shell binding energy reaches the pair-production threshold (E1sb∼2mc2), a shift of +11.0 keV is found. This shift is almost cancelled by the vacuum polarization, leaving a negligible effect for all quantum-electrodynamical corrections of order α but all orders of Zα.
Abschließend sollen hier die wichtigsten, neuen Ergebnisse herausgestellt und ein Ausblick auf mögliche zukünftige Studien gegeben werden. In dieser Arbeit wurden vorwiegend Schwerionenkollisionen bei Einschußenergien zwischen ungefähr 40 MeV/Nukleon und 400 MeV/Nukleon mit dem Quantenmolekulardynamik-Modell untersucht. Ein Schwerpunkt war hierbei die Beschreibung der Umkehr des kollektiven, transversalen Seitwärtsflusses in der Reaktionsebene. Der negative Seitwärtsfluß, der bei niedrigen Energien der Größenordnung kleiner als 100 MeV/Nukleon durch die attraktiven Wechselwirkungen verursacht wird, verschwindet bei Steigerung der Einschußenergie bei der Balance-Energie E-bal. einsetzt. Oberhalb dieser dominieren die repulsiven Wechselwirkungen, so daß positiver transversaler Fluß einsetzt. Sowohl die negativen Flußwinkel als auch der Übergang hin zu positiven Flußwinkeln konnte fur eine große Anzahl verschiedener Energien und Stoßparameter mit unterschiedlichen Zustandsgleichungen für die Systeme 40-20-Ca + 40-20-Ca und 197-79 Au + 197-79 Au mit dem Quantenmolekulardynamik-Modell beschrieben werden. Ziel muß es bleiben, die verschiedenen, grundlegenden physikalischenWechselwirkungen eindeutig und unabhängig voneinander zu bestimmen. Ein erfolgversprechender Weg sind die hier vorgestellten Methoden und die Hinweise zur ad quaten Interpretation experimenteller Ergebnisse. Die Abhängigkeit der Balance-Energien von der Masse des betrachteten Systems ist sehr sensitiv auf den Nukleon-Nukleon Wirkungsquerschnitt im Medium. Hier wurde systematisch gezeigt, daß die Balance-Energien stark vom Stoßparameter abhängen. Die Zunahme der Balance-Energie mit dem Stoßparameter ist ungefähr linear. Für das System Ca+Ca kann sich die Balance-Energie beim Übergang von zentraleren zu mittleren Stoßparametern mehr als verdoppeln. Daher ist für die Interpretation der gemessenen Balance-Energien in bezug auf eine Modifikation des nukleo- nischen Wirkungsquerschnitts im Medium oder der Zustandsgleichung eine genaue Kenntnis des Stoßparameters von größter Wichtigkeit. Vorläufige experimentelle Analysen scheinen die vorhergesagte Stoßparameterabhängigkeit sehr gut zu bestätigen [Wes 95]. Weiterhin hat sich herauskristallisiert, daß bei der Berücksichtigung impulsabhängiger Wechselwirkungen die Balance-Energien bei größeren Stoßparametern signifikant kleiner sind als für den Fall der Nichtberücksichtung. Daher konnten experimentelle Bestimmungen der Balance- Energien bei größeren Stoßparametern signifikante Hinweise auf die tatsächliche Bedeutung der impulsabhängigen Wechselwirkungen in diesem Energiebereich geben. Es wurde gezeigt, daß für schwere Systeme wie Au+Au die langreichweitige internukleare Coulomb-Wechselwirkung vor dem Kontakt der Kerne im Energiebereich der Balance-Energien nicht vernachlässigt werden darf. Die hervorgerufene Repulsion bewirkt eine Drehung des Systems. Während in diesem gedrehten System dynamischer negativer Fluß beobachtbar ist, ist er es nicht im Laborsystem. Die im gedrehten Kontaktbezugssystem bestimmten Balance- Energien fur Au+Au sind erwartungsgemäß kleiner als für Ca+Ca und nehmen mit wachsendem Stoßparameter zu. Ein neuartiger Zwei-Komponenten-Fluß konnte in semiperipheren Kollisionen von Ca+Ca be- schrieben und analysiert werden. Dabei wird in einem Ereignis in verschiedenen Rapiditätsbereichen gleichzeitig positiver und negativer transversaler Fluß möglich. Die wenig komprimierte Spektatorenmaterie, die vermehrt aus schwereren Fragmenten besteht, zeigt negativen Fluß bei großen Rapiditäten, wohingegen dieKompressionszone in Form von einzelnen Nukleonen positiven transversalen Fluß zeigt. Aufgrund der großen Sensitivität gegenüber den Systemparametern und der Zustandsgleichung lohnt es sich, diesen Effekt experimentell zu untersuchen. Beim Studium azimuthaler Verteilungen wurde deutlich, daß auch in den Balance-Punkten noch kollektiver Fluß in Form von azimuthaler Asymmetrie vorliegt. Im Gegensatz zur bekannten hochenergetischen Bevorzugung der Emissionswinkel senkrecht zur Reaktionsebene für Teilchen aus der Wechselwirkungszone wurde hier die bei kleineren Energien preferentielle Emission in die Reaktionsebene aufgezeigt. Diese nimmt mit der Teilchenmasse und dem Stoßparameter zu. Das systematische Studium der Anregungsfunktion dieser azimuthalen Asymmetrie könnte durch die Übergangsenergien, die durch den Wechsel von der preferentiellen Emission in die Reaktionsebene zu der Bevorzugung der Winkel senkrecht zur Reaktionsebene definiert sind, wertvolle, ergänzende Information zu den Balance-Energien liefern.
Invited talk at the 7th International Conference on Strangeness in Quark Matter, SQM 2003, Atlantic Beach, North Carolina, USA, 12-17 Mar, 2003. 11 pages, 12 figures. Journal-ref: J.Phys. G30 (2004) S139-S150. We review recent developments in the field of microscopic transport model calculations for ultrarelativistic heavy ion collisions. In particular, we focus on the strangeness production, for example, the phi-meson and its role as a messenger of the early phase of the system evolution. Moreover, we discuss the important e ects of the (soft) field properties on the multiparticle system. We outline some current problems of the models as well as possible solutions to them
Invited talk at the XXXIII International Symposium on Multiparticle Dynamics, Krakow, Poland, 5-11 Sept, 2003. 5 pages, 1 figure Journal-ref: Acta Phys.Polon. B35 (2004) 23-28. We review the recent developments on microscopic transport calculations for two-particle correlations at low relative momenta in ultrarelativistic heavy ion collisions at RHIC.
Invited talk at the International Workshop XXX on Gross Properties of Nuclei and Nuclear Excitations - Ultrarelativistic Heavy-Ion Collisions, Jan. 13-19, 2002, Hirschegg, Austria. Report-no: LBNL-49674. We discuss predictions for the pion and kaon interferometry measurements in relativistic heavy ion collisions at SPS and RHIC energies. In particular, we confront relativistic transport model calculations that include explicitly a first-order phase transition from a thermalized quark-gluon plasma to a hadron gas with recent data from the RHIC experiments. We critically examine the "HBT-puzzle" both from the theoretical as well as from the experimental point of view. Alternative scenarios are briefly explained.
The centrality dependence of (multi-)strange hadron abundances is studied for Pb(158 AGeV)Pb reactions and compared to p(158 GeV)Pb collisions. The microscopic transport model UrQMD is used for this analysis. The predicted Lambda/pi-, Xi-/pi- and Omega-/pi- ratios are enhanced due to rescattering in central Pb-Pb collisions as compared to peripheral Pb-Pb or p-Pb collisions. A reduction of the constituent quark masses to the current quark masses m_s \sim 230 MeV, m_q \sim 10 MeV, as motivated by chiral symmetry restoration, enhances the hyperon yields to the experimentally observed high values. Similar results are obtained by an ad hoc overall increase of the color electric field strength (effective string tension of kappa=3 GeV/fm). The enhancement depends strongly on the kinematical cuts. The maximum enhancement is predicted around midrapidity. For Lambda's, strangeness suppression is predicted at projectile/target rapidity. For Omega's, the predicted enhancement can be as large as one order of magnitude. Comparisons of Pb-Pb data to proton induced asymmetric (p-A) collisions are hampered due to the predicted strong asymmetry in the various rapidity distributions of the different (strange) particle species. In p-Pb collisions, strangeness is locally (in rapidity) not conserved. The present comparison to the data of the WA97 and NA49 collaborations clearly supports the suggestion that conventional (free) hadronic scenarios are unable to describe the observed high (anti-)hyperon yields in central collisions. The doubling of the strangeness to nonstrange suppression factor, gamma_s \approx 0.65, might be interpreted as a signal of a phase of nearly massless particles.
Directed and elliptic flow
(1999)
We compare microscopic transport model calculations to recent data on the directed and elliptic flow of various hadrons in 2 - 10 A GeV Au+Au and Pb (158 A GeV) Pb collisions. For the Au+Au excitation function a transition from the squeeze-out to an in-plane enhanced emission is consistently described with mean field potentials corresponding to one incompressibility. For the Pb (158 A GeV) Pb system the elliptic flow prefers in-plane emission both for protons and pions, the directed flow of protons is opposite to that of the pions, which exhibit anti-flow. Strong directed transverse flow is present for protons and Lambdas in Au (6 A GeV) Au collisions as well. Both for the SPS and the AGS energies the agreement between data and calculations is remarkable.
We calculate the Gaussian radius parameters of the pion-emitting source in high energy heavy ion collisions, assuming a first order phase transition from a thermalized Quark-Gluon-Plasma (QGP) to a gas of hadrons. Such a model leads to a very long-lived dissipative hadronic rescattering phase which dominates the properties of the two-pion correlation functions. The radii are found to depend only weakly on the thermalization time tau i, the critical temperature T c (and thus the latent heat), and the specific entropy of the QGP. The dissipative hadronic stage enforces large variations of the pion emission times around the mean. Therefore, the model calculations suggest a rapid increase of R out/R side as a function of K T if a thermalized QGP were formed.
We make predictions for the kaon interferometry measurements in Au+Au collisions at the Relativistic Heavy Ion Collider (RHIC). A first order phase transition from a thermalized Quark-Gluon-Plasma (QGP) to a gas of hadrons is assumed for the transport calculations. The fraction of kaons that are directly emitted from the phase boundary is considerably enhanced at large transverse momenta K T ~ 1 GeV/c. In this kinematic region, the sensitivity of the R out/R side ratio to the QGP-properties is enlarged. Here, the results of the 1-dimensional correlation analysis are presented. The extracted interferometry radii, depending on K-Theta, are not unusually large and are strongly affected by momentum resolution effects.