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Electron–phonon coupling and electron–phonon scattering in SrVO3

  • Understanding the physics of strongly correlated electronic systems has been a central issue in condensed matter physics for decades. In transition metal oxides, strong correlations characteristic of narrow d bands are at the origin of remarkable properties such as the opening of Mott gap, enhanced effective mass, and anomalous vibronic coupling, to mention a few. SrVO3 with V4+ in a 3d1 electronic configuration is the simplest example of a 3D correlated metallic electronic system. Here, the authors' focus on the observation of a (roughly) quadratic temperature dependence of the inverse electron mobility of this seemingly simple system, which is an intriguing property shared by other metallic oxides. The systematic analysis of electronic transport in SrVO3 thin films discloses the limitations of the simplest picture of e–e correlations in a Fermi liquid (FL); instead, it is shown show that the quasi-2D topology of the Fermi surface (FS) and a strong electron–phonon coupling, contributing to dress carriers with a phonon cloud, play a pivotal role on the reported electron spectroscopic, optical, thermodynamic, and transport data. The picture that emerges is not restricted to SrVO3 but can be shared with other 3d and 4d metallic oxides.
Metadaten
Author:Mathieu MirjoletORCiD, Francisco RivadullaORCiD, Premysl MarsikORCiD, Vladislav BorisovORCiD, Roser ValentíORCiDGND, Josep FontcubertaORCiD
URN:urn:nbn:de:hebis:30:3-723106
DOI:https://doi.org/10.1002/advs.202004207
ISSN:2198-3844
ArXiv Id:http://arxiv.org/abs/2105.01579
Parent Title (English):Advanced science
Publisher:Wiley-VCH
Place of publication:Weinheim
Document Type:Article
Language:English
Date of Publication (online):2021/06/19
Date of first Publication:2021/06/19
Publishing Institution:Universitätsbibliothek Johann Christian Senckenberg
Release Date:2024/02/20
Tag:electron–phonon coupling; polarons; quadratic temperature dependent resistivity; strongly correlated electrons; strontium vanadate epitaxial films; vanadium oxides
Volume:8
Issue:15, art. 2004207
Article Number:2004207
Page Number:12
First Page:1
Last Page:12
Institutes:Physik
Dewey Decimal Classification:5 Naturwissenschaften und Mathematik / 53 Physik / 530 Physik
5 Naturwissenschaften und Mathematik / 54 Chemie / 540 Chemie und zugeordnete Wissenschaften
6 Technik, Medizin, angewandte Wissenschaften / 60 Technik / 600 Technik, Technologie
6 Technik, Medizin, angewandte Wissenschaften / 62 Ingenieurwissenschaften / 620 Ingenieurwissenschaften und zugeordnete Tätigkeiten
Sammlungen:Universitätspublikationen
Licence (German):License LogoCreative Commons - CC BY - Namensnennung 4.0 International